Coherent Optical Parallel Computing

Livrables

Best procedures of functionalization/assembly

Final report on best procedure for functionalization and assembly suitable for WP3 and WP4. (M42 P4, P2-YP, P3, P5, P7)

Surface functionalization procedures

Report on surface functionalization procedures (M20, P4, P2-YP)

Applied theory of computing by observables

Applied theory of computing by observables and long time stability (M36, P2-RL, P1, P3-BF, P6).

Design and modelling of prototype

Report on prototype modelling and design (M12, P5,P7, P4, P2-YP,P3-EC,P1, P2-RDL)

Technological roadmap

Technological roadmap (M42, P7).

Demonstration of parallel logic

Demonstration of parallel logic for distinct units operating in parallel (M24), on arrays (M42) in a single and in several phase matching directions (P3-BF with P1, P2-RL).

QD and core-shell nanostructure synthesis

Report on procedures for the synthesis of QDs and core-shell with defined optical properties (M12, P4)

Layered structures with high delocalization

Fabricating a layered structure exhibiting nearest neighbor electronic delocalization at ambient conditions. (M24, P2-YP, P4)

Multiscale modelling and model Hamiltonians

Multiscale modelling and model Hamiltonians of organic dyes (M12) and arrays SC- QDs (M24) for feedback to WPs2&3, and for guiding data interpretation in WP3 (P1, P2-RL, P3-BF).

All PM directions optical response simulations

Simulation of the optical response in all phase matching directions of dyes (M18), arrays of SC- QDs (M36), and comparison with experimental spectra of P3-EC, in the perturbative limit (P3-BF) and to higher orders (P1, P2-RL).

Scientific and Technical progress Report
Theory of compiler targeting PMVL machines and virtual experiments

Report on the theory of compiler targeting PLMV machine (M18) and virtual experiment (M30) P6, P1, P2-RL How PLMV functions could be use as instruction set and how they could be used to implement compound operations.

Complete set of 2D data on multichromophoric systems and on arrays

Complete set of 2D data on multi-chromophoric systems (networks of nanosystems) in solution (M30, P3-EC) and embedded in solid state matrices to characterized the inter unit coupling dynamics. (M24, P3-EC)

Compiler targeting realistic PMVL machines

Compiler targeting realistic PMLV machine A software simulator of feasible machine and compilers targeting this machine will be provided as well as program examples (M36, P6, P1, P2-RL).

Complete set of 2D data on solutions

Complete set of 2D data on solutions of organic dyes, SC-QD and dimers thereof to establish a correspondence between experimental results and logic operations. (M12, P3-EC).

System design

Report of system design (M42, P7, all)

Multiphase matching experiment data set on complex systems

Multi-phase matching experiment dataset on complex systems (M42, P3-EC) and implications to logic synthesis and architecture and device integration.

Dissemination and Exploitation plan

Dissemination and Exploitation plan (M12, P6)

Website

COPAC project website (restricted (P1) and public (P6), regularly updated) and a logo.

Data management plan

Data Management plan, (M6, P1)

Publications

Coupling effects in QD dimers at sub-nanometer interparticle distance

Auteurs: Carlo Nazareno Dibenedetto, Elisabetta Fanizza, Rosaria Brescia, Yuval Kolodny, Sergei Remennik, Annamaria Panniello, Nicoletta Depalo, Shira Yochelis, Roberto Comparelli, Angela Agostiano, Maria Lucia Curri, Yossi Paltiel, Marinella Striccoli
Publié dans: Nano Research, Numéro 13/4, 2020, Page(s) 1071-1080, ISSN 1998-0124
Éditeur: Tsinghua Univ Press
DOI: 10.1007/s12274-020-2747-3

Tuning Quantum Dots Coupling Using Organic Linkers with Different Vibrational Modes

Auteurs: Yuval Kolodny, Stav Fererra, Veniamin Borin, Shira Yochelis, Carlo Nazareno Dibenedetto, Morin Mor, Joanna Dehnel, Sergei Remmenik, Elisabetta Fanizza, Marinella Striccoli, Igor Schapiro, Efrat Lifshitz, Yossi Paltiel
Publié dans: The Journal of Physical Chemistry C, Numéro 124/29, 2020, Page(s) 16159-16165, ISSN 1932-7447
Éditeur: American Chemical Society
DOI: 10.1021/acs.jpcc.0c03703

Massively parallel classical logic via coherent dynamics of an ensemble of quantum systems with dispersion in size.

Auteurs: Hugo Gattuso; Raphael D. Levine; Raphael D. Levine; Françoise Remacle; Françoise Remacle
Publié dans: Proc Natl Acad Sci U S A, Numéro 4, 2020, ISSN 1091-6490
Éditeur: National Academy of Science
DOI: 10.26434/chemrxiv.12370538.v1

Quantum Device Emulates the Dynamics of Two Coupled Oscillators

Auteurs: Ksenia Komarova, Hugo Gattuso, R. D. Levine, F. Remacle
Publié dans: The Journal of Physical Chemistry Letters, Numéro 11/17, 2020, Page(s) 6990-6995, ISSN 1948-7185
Éditeur: American Chemical Society
DOI: 10.1021/acs.jpclett.0c01880

Chirality of a rhodamine heterodimer linked to a DNA scaffold: an experimental and computational study

Auteurs: P. S. Rukin, K. G. Komarova, B. Fresch, E. Collini, F. Remacle
Publié dans: Physical Chemistry Chemical Physics, Numéro 22/14, 2020, Page(s) 7516-7523, ISSN 1463-9076
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d0cp00223b

Quantum Phenomena in Nanomaterials: Coherent Superpositions of Fine Structure States in CdSe Nanocrystals at Room Temperature

Auteurs: Elisabetta Collini, Hugo Gattuso, Luca Bolzonello, Andrea Casotto, Andrea Volpato, Carlo Nazareno Dibenedetto, Elisabetta Fanizza, Marinella Striccoli, Françoise Remacle
Publié dans: The Journal of Physical Chemistry C, Numéro 123/51, 2019, Page(s) 31286-31293, ISSN 1932-7447
Éditeur: American Chemical Society
DOI: 10.1021/acs.jpcc.9b11153

Time resolved mechanism of the isotope selectivity in the ultrafast light induced dissociation in N 2

Auteurs: Ksenia G. Komarova, Francoise Remacle, R. D. Levine
Publié dans: The Journal of Chemical Physics, Numéro 151/11, 2019, Page(s) 114308, ISSN 0021-9606
Éditeur: American Institute of Physics
DOI: 10.1063/1.5118990

Photocurrent-Detected 2D Electronic Spectroscopy Reveals Ultrafast Hole Transfer in Operating PM6/Y6 Organic Solar Cells

Auteurs: Luca Bolzonello, Francisco Bernal-Texca, Luis G. Gerling, Jana Ockova, Elisabetta Collini, Jordi Martorell, Niek F. van Hulst
Publié dans: The Journal of Physical Chemistry Letters, Numéro 12/16, 2021, Page(s) 3983-3988, ISSN 1948-7185
Éditeur: American Chemical Society
DOI: 10.1021/acs.jpclett.1c00822

Parallel Quantum Computation of Vibrational Dynamics

Auteurs: Ksenia Komarova; Hugo Gattuso; R. D. Levine; R. D. Levine; R. D. Levine; F. Remacle; F. Remacle
Publié dans: Frontiers in Physcis, Numéro 4, 2020, ISSN 2296-424X
Éditeur: Frontiers
DOI: 10.26434/chemrxiv.12814793

Room-Temperature Inter-Dot Coherent Dynamics in Multilayer Quantum Dot Materials

Auteurs: Elisabetta Collini, Hugo Gattuso, Yuval Kolodny, Luca Bolzonello, Andrea Volpato, Hanna T. Fridman, Shira Yochelis, Morin Mor, Johanna Dehnel, Efrat Lifshitz, Yossi Paltiel, Raphael D. Levine, Françoise Remacle
Publié dans: The Journal of Physical Chemistry C, Numéro 124/29, 2020, Page(s) 16222-16231, ISSN 1932-7447
Éditeur: American Chemical Society
DOI: 10.1021/acs.jpcc.0c05572

Coherent Exciton Dynamics in Ensembles of Size-Dispersed CdSe Quantum Dot Dimers Probed via Ultrafast Spectroscopy: A Quantum Computational Study

Auteurs: Hugo Gattuso, Barbara Fresch, Raphael D. Levine, Françoise Remacle
Publié dans: Applied Sciences, Numéro 10/4, 2020, Page(s) 1328, ISSN 2076-3417
Éditeur: mdpi
DOI: 10.3390/app10041328

Spectral shift, electronic coupling and exciton delocalization in nanocrystal dimers: insights from all-atom electronic structure computations

Auteurs: Maurizio Coden, Pietro De Checchi, Barbara Fresch
Publié dans: Nanoscale, Numéro 12/35, 2020, Page(s) 18124-18136, ISSN 2040-3364
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d0nr05601d

Deciphering hot- and multi-exciton dynamics in core–shell QDs by 2D electronic spectroscopies

Auteurs: Marcello Righetto, Luca Bolzonello, Andrea Volpato, Giordano Amoruso, Annamaria Panniello, Elisabetta Fanizza, Marinella Striccoli, Elisabetta Collini
Publié dans: Physical Chemistry Chemical Physics, Numéro 20/27, 2018, Page(s) 18176-18183, ISSN 1463-9076
Éditeur: Royal Society of Chemistry
DOI: 10.1039/c8cp02574f

Optimization and selection of time-frequency transforms for wave-packet analysis in ultrafast spectroscopy

Auteurs: Andrea Volpato, Elisabetta Collini
Publié dans: Optics Express, Numéro 27/3, 2019, Page(s) 2975, ISSN 1094-4087
Éditeur: Optical Society of America
DOI: 10.1364/OE.27.002975

Characterization of the coherent dynamics of bacteriochlorophyll a in solution

Auteurs: Elena Meneghin, Danilo Pedron, Elisabetta Collini
Publié dans: Chemical Physics, Numéro 519, 2019, Page(s) 85-91, ISSN 0301-0104
Éditeur: Elsevier BV
DOI: 10.1016/j.chemphys.2018.12.008

Spectroscopy data for the time and frequency characterization of vibrational coherences in bacteriochlorophyll a

Auteurs: Elena Meneghin, Danilo Pedron, Elisabetta Collini
Publié dans: Data in Brief, Numéro 23, 2019, Page(s) 103707, ISSN 2352-3409
Éditeur: Elsevier BV
DOI: 10.1016/j.dib.2019.103707

Effect of Different Conformational Distributions on the Ultrafast Coherence Dynamics in Porphyrin-Based Polymers

Auteurs: Andrea Volpato, Mirco Zerbetto, Luca Bolzonello, Elena Meneghin, Barbara Fresch, Tiziana Benelli, Loris Giorgini, Elisabetta Collini
Publié dans: The Journal of Physical Chemistry C, Numéro 123/16, 2019, Page(s) 10212-10224, ISSN 1932-7447
Éditeur: American Chemical Society
DOI: 10.1021/acs.jpcc.8b12562

Fast Energy Transfer in CdSe Quantum Dot Layered Structures: Controlling Coupling with Covalent-Bond Organic Linkers

Auteurs: Eyal Cohen, Pavel Komm, Noa Rosenthal-Strauss, Joanna Dehnel, Efrat Lifshitz, Shira Yochelis, Raphael D. Levine, Francoise Remacle, Barbara Fresch, Gilad Marcus, Yossi Paltiel
Publié dans: The Journal of Physical Chemistry C, Numéro 122/10, 2018, Page(s) 5753-5758, ISSN 1932-7447
Éditeur: American Chemical Society
DOI: 10.1021/acs.jpcc.7b11799

Spin-Exciton Delocalization Enhancement in Multilayer Chiral Linker/Quantum Dot Structures

Auteurs: Hanna T. Fridman, Johanna Dehnel, Shira Yochelis, Efrat Lifshitz, Yossi Paltiel
Publié dans: The Journal of Physical Chemistry Letters, Numéro 10/14, 2019, Page(s) 3858-3862, ISSN 1948-7185
Éditeur: American Chemical Society
DOI: 10.1021/acs.jpclett.9b01433

Quantum Dot Coupling in a Vertical Transport Device under Ambient Conditions

Auteurs: Aviya Perlman Illouz, Eyal Cohen, Uri Peskin, Shira Yochelis, Yossi Paltiel
Publié dans: ACS Omega, Numéro 3/6, 2018, Page(s) 6224-6229, ISSN 2470-1343
Éditeur: ACS
DOI: 10.1021/acsomega.8b00867

Coupling in quantum dot molecular hetero-assemblies

Auteurs: Carlo Nazareno Dibenedetto, Elisabetta Fanizza, Liberato De Caro, Rosaria Brescia, Annamaria Panniello, Raffaele Tommasi, Chiara Ingrosso, Cinzia Giannini, Angela Agostiano, Maria Lucia Curri, Marinella Striccoli
Publié dans: Materials Research Bulletin, Numéro 146, 2022, Page(s) 111578, ISSN 0025-5408
Éditeur: Pergamon Press Ltd.
DOI: 10.1016/j.materresbull.2021.111578

Ultrafast fs coherent excitonic dynamics in CdSe quantum dots assemblies addressed and probed by 2D electronic spectroscopy

Auteurs: Elisabetta Collini, Hugo Gattuso, R. D. Levine, F. Remacle
Publié dans: The Journal of Chemical Physics, Numéro 154/1, 2021, Page(s) 014301, ISSN 0021-9606
Éditeur: American Institute of Physics
DOI: 10.1063/5.0031420

Surprisal of a Quantum State: Dynamics, Compact Representation and Coherence Effects

Auteurs: K. Komarova; F. Remacle; R. D. Levine
Publié dans: Surprisal of a quantum state: Dynamics, compact representation, and coherence effects. <i>The Journal of Chemical Physics, 153</i>(21), 214105. (2020)., Numéro 4, 2020, ISSN 0021-9606
Éditeur: American Institute of Physics
DOI: 10.26434/chemrxiv.12981857.v1

Lasers pumped quantum dynamics in nanostructured arrays for computing

Auteurs: Ariela Donval, Noam Gross, Moshe Oron
Publié dans: Quantum Information Science, Sensing, and Computation X, 2018, Page(s) 4, ISBN 9781-510618329
Éditeur: SPIE
DOI: 10.1117/12.2299961

Computing using quantum dynamics of nanostructured arrays

Auteurs: Noam Gross, Ariela Donval
Publié dans: Quantum Information Science, Sensing, and Computation XI, 2019, Page(s) 2, ISBN 9781-510626348
Éditeur: SPIE
DOI: 10.1117/12.2518299

An n-bit adder realized via coherent optical parallel computing

Auteurs: Bogdan Reznychenko, Emmanuel Mazer, Maurizio Coden, Elisabetta Collini, Carlo Nazareno DiBenedetto, Ariela Donval, Barbara Fresch, Hugo Gattuso, Noam Gross, Yossi Paltiel, Francoise Remacle, Marinella Striccoli
Publié dans: 2019 IEEE International Conference on Rebooting Computing (ICRC), 2019, Page(s) 146-152, ISBN 978-1-7281-5221-9
Éditeur: IEEE eXpress Conference Publishing

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