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Soap Film based Artificial Photosynthesis

CORDIS proporciona enlaces a los documentos públicos y las publicaciones de los proyectos de los programas marco HORIZONTE.

Los enlaces a los documentos y las publicaciones de los proyectos del Séptimo Programa Marco, así como los enlaces a algunos tipos de resultados específicos, como conjuntos de datos y «software», se obtienen dinámicamente de OpenAIRE .

Resultado final

Multi-physics model of soap-film in COMSOL environment (se abrirá en una nueva ventana)

Multiphysics model of soapfilm in COMSOL environment

Article on transfer reactions in Soap Film (se abrirá en una nueva ventana)
1st update of Dissemination and Exploitation plan (se abrirá en una nueva ventana)
Article on properties of dis-symmetric soap film as an AP membrane (se abrirá en una nueva ventana)

Article on properties of dissymmetric soap film as an AP membrane

Article on the molecular structure of the water-CO2 AP interface (se abrirá en una nueva ventana)

Article on the molecular structure of the waterCO2 AP interface

Debugged code for fluidic optimization (se abrirá en una nueva ventana)
Techno-economic report on AP (se abrirá en una nueva ventana)

Technoeconomic report on AP

Database of transport coefficient in Matlab environment (se abrirá en una nueva ventana)

Database of transport coefficient in Matlab environment. Main modelling results will be disseminated through the European Materials Modelling Council ensuring wide research visibility.

2nd update of Dissemination and Exploitation plan (se abrirá en una nueva ventana)
Dissemination and Exploitation plan (se abrirá en una nueva ventana)

A draft “plan for the dissemination and exploitation” (D6.2) is presented below: Actions taken according to this plan will be updated periodically (M12, M30, M42) by tracking & monitoring key performance indicators (KPIs). Dissemination to Scientific Community: Interdisciplinary results will be communicated to diverse peer groups. The leadership of key SoFiA members in national AP platforms is already established (UK Solar Fuels Network, Swedish AP consortium) and will facilitate networking and community building with other interested members. Data management Plan (DMP): SoFiA will participate in the Pilot on Open Research Data and will provide open access to raw data corresponding to modelling & simulation, as well as data required to reproduce the results presented in scientific publications. These data will be stored in Zenodo (a research data repository created by CERN) ensuring their public availability and long-time preservation. Details will be provided in a data management plan (DMP, D5.3), to be delivered by M6 and updated periodically (M12, M30). Main modelling results will be disseminated through the European Materials Modelling Council ensuring wide research visibility. Publications: We will prioritise Gold or Green (with 6 months embargo) open access publication. At least 8 publications are estimated in journals with the highest impact in multidisciplinary science, in materials sciences, in nanotechnology, and in chemistry. KPI- Impact factor of accepted journals, citations, author h-index. Course Materials, Conferences & Workshops: In June 2020, our partner ICTP (UNESCO flagship institute) will host Conference on the Complex Interactions of Light and Biological Matter: Experiments meet Theory. We will organize in a special AP session showcasing our project through posters and oral communications and will host a workshop and an information kiosk dedicated to SoFiA. A summer school for PhD students, on AP will be organized and hosted by UU (by M30) Our start-up executive body WI (non-beneficiary) is supported by Sofia Tech Park (STP) - a (Bulgarian flagship) EU project. With support of WI and STP we will host a workshop (by M46) on solar fuels with focus on AP in Bulgaria (energetically poor/unsustainable region), and tailored for an audience usually remote from the EU policy dialogue. All partners will attend the most relevant conferences (including MRS, ACS, ISF, etc.). SoFiA will also participate in the annual FET Conferences. Our IPR protected findings, concept design and selected experimental results will be included as graduate level course material at partner Universities. Course update plans will be included as chapters in final two project periodic reports on M30 & M48. KPI- Attendance in Summer School, Workshop, and attendee/student feedback. Related EU projects will be monitored and contacted. Key representatives will be invited for lectures at the Bulgaria workshop. SoFiA will enhance networking possibilities with the following programs: FET projects – A-Leaf (Proactive) and Diacat (Open), from ERC Grantees in AP (COFLeaf; ENLIGHT; HyMAP; HYMEM; photocatH2ode; TripleSolar; and others.) KPI- New collaborations for Phase II, III and feedback from AP experts. Dissemination to Industrial sector and to Policy Makers- SoFiA will participate in relevant industrial fairs, for instance: SSIS (smart systems industry summit), W3+FAIR. For critical coverage of breakthrough results we have identified policy journals: ENDS Europe, and Brussels based Politico and Euractiv. To communicate with EU policymakers, the coordinator will contact OBSERVE- a FET-CSA that supports Europe in FET, and FET2RIN, a network connecting FET projects to potential investors. Through EAB meetings, IPR protected research findings will be communicated to Shell, Air Liquide and Unilever who are interested in commercial exploitation. Climate & Policy experts at EAB will be consulted to indicate policy hook for market uptake. EAB feedback

Final update of Dissemination and Exploitation plan (se abrirá en una nueva ventana)
Project website with open and restricted access (se abrirá en una nueva ventana)

Project website & social media networking will be set up by M2 (D5.1) and updated on a monthly basis. We have a logo. Website will include news & events, links to partners’ websites, a press desk, publications, and search functionalities. The website will also promote important (public) results from related projects in AP and will administer an open forum as a knowledge-sharing tool for partners and user communities. Facebook, Twitter and LinkedIn will be used to promote the website content. An impact assessment of the entire social media communications activities will be carried out by monitoring web hits, likes, followers, retweets (KPI). Videos & news bytes will also be promoted through Hassim Al-Ghaili’s science communication website which has >16M fans. The existing Wikipedia page on AP will be updated with critical results from SoFiA.

Final update of Data management plan (se abrirá en una nueva ventana)
2nd update of Data management plan (se abrirá en una nueva ventana)
Data management plan (se abrirá en una nueva ventana)

Data management Plan (DMP): SoFiA will participate in the Pilot on Open Research Data and will provide open access to raw data corresponding to modelling & simulation, as well as data required to reproduce the results presented in scientific publications. These data will be stored in Zenodo (a research data repository created by CERN) ensuring their public availability and long-time preservation. Details will be provided in a data management plan (DMP, D6.3), to be delivered by M6 and updated periodically (M12, M30). Main modelling results will be disseminated through the European Materials Modelling Council ensuring wide research visibility. Publications: We will prioritise Gold or Green (with 6 months embargo) open access publication. At least 8 publications are estimated in journals with the highest impact in multidisciplinary science, in materials sciences, in nanotechnology, and in chemistry. KPI- Impact factor of accepted journals, citations, author h-index.

Publicaciones

Shorter Alkyl Chains Enhance Molecular Diffusion and Electron Transfer Kinetics between Photosensitisers and Catalysts in CO 2 -Reducing Photocatalytic Liposomes. (se abrirá en una nueva ventana)

Autores: David M. Klein; Santiago Rodríguez-Jiménez; Marlene E. Hoefnagel; Andrea Pannwitz; Andrea Pannwitz; Amrutha Prabhakaran; Maxime A. Siegler; Tia E. Keyes; Erwin Reisner; Albert M. Brouwer; Sylvestre Bonnet
Publicado en: Chem.Eur.J., Edición 2021, 27, 2021, Página(s) 17203–17212, ISSN 0947-6539
Editor: John Wiley & Sons Ltd.
DOI: 10.1002/chem.202102989

A novel concept of photosynthetic soft membranes: a numerical study (se abrirá en una nueva ventana)

Autores: Gabriele Falciani, Luca Bergamasco, Shannon A. Bonke, Indraneel Sen, Eliodoro Chiavazzo
Publicado en: Discover nano, 2023, Página(s) 15, ISSN 2731-9229
Editor: Springer Nature
DOI: 10.1186/s11671-023-03772-1

Realizing Symmetry-Breaking Architectures in Soap Films (se abrirá en una nueva ventana)

Autores: Nidhi Kaul, Luca Bergamasco, Hongwei Song, Thijs Varkevisser, Agnese Amati, Gabriele Falciani, Cees J. M. van Rijn, Eliodoro Chiavazzo, Indraneel Sen, Sylvestre Bonnet, Leif Hammarström
Publicado en: Physical Review Letters, Edición 132, 2024, ISSN 0031-9007
Editor: American Physical Society
DOI: 10.1103/physrevlett.132.028201

Interfacial Characterization of Ruthenium-Based Amphiphilic Photosensitizers (se abrirá en una nueva ventana)

Autores: Yousra Timounay, Andrea Pannwitz, David M. Klein, Anne-Laure Biance, Marlene E. Hoefnagel, Indraneel Sen, Alain Cagna,* Marie Le Merrer,* and Sylvestre Bonnet*
Publicado en: Langmuir, Edición 38, 2022, 2022, Página(s) 9697-9707, ISSN 0743-7463
Editor: American Chemical Society
DOI: 10.1021/acs.langmuir.2c01391

Water-Induced Restructuring of the Surface of a Deep Eutectic Solvent (se abrirá en una nueva ventana)

Autores: Rahul Gera, Carolyn J. Moll, Aditi Bhattacherjee, Huib J. Bakker
Publicado en: The Journal of Physical Chemistry Letters, Edición 13, 2023, Página(s) 634-641, ISSN 1948-7185
Editor: American Chemical Society
DOI: 10.1021/acs.jpclett.1c03907

Multi-Variable Multi-Metric Optimisation of Self-Assembled Photocatalytic CO2 Reduction Performance using Machine Learning Algorithms (se abrirá en una nueva ventana)

Autores: Shannon Bonke, Giovanni Trezza, Luca Bergamasco, Hongwei Song, Santiago Rodríguez-Jiménez, Leif Hammarström, Eliodoro Chiavazzo, Erwin Reisner
Publicado en: Journal of the Americal Chemical Society, 2023, ISSN 0002-7863
Editor: American Chemical Society
DOI: 10.26434/chemrxiv-2023-g5hkm

Molecularly engineered photocatalyst sheet for scalable solar formate production from carbon dioxide and water (se abrirá en una nueva ventana)

Autores: Qian Wang, Julien Warnan, Santiago Rodríguez-Jiménez, Jane J. Leung, Shafeer Kalathil, Virgil Andrei, Kazunari Domen, Erwin Reisner
Publicado en: Nature Energy, 2020, ISSN 2058-7546
Editor: Nature
DOI: 10.1038/s41560-020-0678-6

Observation of Strong Synergy in the Interfacial Water Response of Binary Ionic and Nonionic Surfactant Mixtures (se abrirá en una nueva ventana)

Autores: Sanghamitra Sengupta, Rahul Gera, Colin Egan, Uriel N. Morzan, Jan Versluis, Ali Hassanali, Huib J. Bakker
Publicado en: The Journal of Physical Chemistry Letters, Edición 13, 2023, Página(s) 11391-11397, ISSN 1948-7185
Editor: American Chemical Society
DOI: 10.1021/acs.jpclett.2c02750

Mechanistic Insights into the Charge Transfer Dynamics of Photocatalytic Water Oxidation at the Lipid Bilayer−Water Interface (se abrirá en una nueva ventana)

Autores: Hongwei Song, Agnese Amati, Andrea Pannwitz, Sylvestre Bonnet, and Leif Hammarström
Publicado en: The Journal of the American Chemical Society, Edición 144, 2022, 2022, Página(s) 19353−19364, ISSN 0002-7863
Editor: American Chemical Society
DOI: 10.1021/jacs.2c06842

Emergence of Electric Fields at the Water–C12E6 Surfactant Interface (se abrirá en una nueva ventana)

Autores: Rahul Gera, Huib J. Bakker, Ricardo Franklin-Mergarejo, Uriel N. Morzan, Gabriele Falciani, Luca Bergamasco, Jan Versluis, Indraneel Sen, Silvia Dante, Eliodoro Chiavazzo, and Ali A. Hassanali
Publicado en: J. Am. Chem. Soc., Edición 2021, 143, 37, 2021, Página(s) 15103–15112, ISSN 0002-7863
Editor: American Chemical Society
DOI: 10.26434/chemrxiv.14661360.v1

Roadmap towards solar fuel synthesis at the water interface of liposome membranes (se abrirá en una nueva ventana)

Autores: A. Pannwitz, D.M. Klein, S. Rodríguez-Jiménez, C. Casadevall, H. Song, E. Reisner, L. Hammarström, S. Bonnet
Publicado en: Chem. Soc. Rev.,, Edición 50, 2021, 2021, Página(s) 4833–4855, ISSN 0306-0012
Editor: Royal Society of Chemistry
DOI: 10.1039/d0cs00737d

An overview on modelling approaches for photochemical and photoelectrochemical solar fuels processes and technologies (se abrirá en una nueva ventana)

Autores: Gabriele Falciani, Eliodoro Chiavazzo
Publicado en: Energy Conversion and Management, 2023, ISSN 0196-8904
Editor: Pergamon Press Ltd.
DOI: 10.1016/j.enconman.2023.117366

Self-Assembled Liposomes Enhance Electron Transfer for Efficient Photocatalytic CO2 Reduction (se abrirá en una nueva ventana)

Autores: "Santiago Rodríguez-Jiménez,# Hongwei Song,# Erwin Lam, Demelza Wright, Andrea Pannwitz, Shannon A. Bonke, Jeremy J. Baumberg, Sylvestre Bonnet, Leif Hammarström,* and Erwin Reisner*"
Publicado en: The Journal of the American Chemical Society, Edición 144, 2022, 2022, Página(s) 9399−9412, ISSN 0002-7863
Editor: American Chemical Society
DOI: 10.1021/jacs.2c01725

Free energy decompositions illuminate synergistic effects in interfacial binding thermodynamics of mixed surfactant systems (se abrirá en una nueva ventana)

Autores: Colin K. Egan, Ali Hassanali
Publicado en: The Journal of Chemical Physics, Edición 159, 2023, ISSN 0021-9606
Editor: American Institute of Physics
DOI: 10.1063/5.0163849

Design and testing of a device for the characterization of gas transfer through soap films and measurement protocol based on color matching (se abrirá en una nueva ventana)

Autores: Gabriele Falciani, Luca Bergamasco, Agnese Amati, Gijsbert Verdoes, Indraneel Sen, Sylvestre Bonnet, Eliodoro Chiavazzo
Publicado en: International Communications in Heat and Mass Transfer, Edición 149, 2023, Página(s) 107161, ISSN 0735-1933
Editor: Pergamon Press Ltd.
DOI: 10.1016/j.icheatmasstransfer.2023.107161

A multi-scale perspective of gas transport through soap-film membranes (se abrirá en una nueva ventana)

Autores: Gabriele Falciani, Ricardo Franklin, Alain Cagna, Indraneel Sen, Ali Hassanali, Eliodoro Chiavazzo
Publicado en: Molecular Systems Design & Engineering, Edición 5/5, 2020, Página(s) 911-921, ISSN 2058-9689
Editor: Royal Society of Chemistry
DOI: 10.1039/c9me00186g

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