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Soap Film based Artificial Photosynthesis

CORDIS fornisce collegamenti ai risultati finali pubblici e alle pubblicazioni dei progetti ORIZZONTE.

I link ai risultati e alle pubblicazioni dei progetti del 7° PQ, così come i link ad alcuni tipi di risultati specifici come dataset e software, sono recuperati dinamicamente da .OpenAIRE .

Risultati finali

Multi-physics model of soap-film in COMSOL environment (si apre in una nuova finestra)

Multiphysics model of soapfilm in COMSOL environment

Article on transfer reactions in Soap Film (si apre in una nuova finestra)
1st update of Dissemination and Exploitation plan (si apre in una nuova finestra)
Article on properties of dis-symmetric soap film as an AP membrane (si apre in una nuova finestra)

Article on properties of dissymmetric soap film as an AP membrane

Article on the molecular structure of the water-CO2 AP interface (si apre in una nuova finestra)

Article on the molecular structure of the waterCO2 AP interface

Debugged code for fluidic optimization (si apre in una nuova finestra)
Techno-economic report on AP (si apre in una nuova finestra)

Technoeconomic report on AP

Database of transport coefficient in Matlab environment (si apre in una nuova finestra)

Database of transport coefficient in Matlab environment. Main modelling results will be disseminated through the European Materials Modelling Council ensuring wide research visibility.

2nd update of Dissemination and Exploitation plan (si apre in una nuova finestra)
Dissemination and Exploitation plan (si apre in una nuova finestra)

A draft “plan for the dissemination and exploitation” (D6.2) is presented below: Actions taken according to this plan will be updated periodically (M12, M30, M42) by tracking & monitoring key performance indicators (KPIs). Dissemination to Scientific Community: Interdisciplinary results will be communicated to diverse peer groups. The leadership of key SoFiA members in national AP platforms is already established (UK Solar Fuels Network, Swedish AP consortium) and will facilitate networking and community building with other interested members. Data management Plan (DMP): SoFiA will participate in the Pilot on Open Research Data and will provide open access to raw data corresponding to modelling & simulation, as well as data required to reproduce the results presented in scientific publications. These data will be stored in Zenodo (a research data repository created by CERN) ensuring their public availability and long-time preservation. Details will be provided in a data management plan (DMP, D5.3), to be delivered by M6 and updated periodically (M12, M30). Main modelling results will be disseminated through the European Materials Modelling Council ensuring wide research visibility. Publications: We will prioritise Gold or Green (with 6 months embargo) open access publication. At least 8 publications are estimated in journals with the highest impact in multidisciplinary science, in materials sciences, in nanotechnology, and in chemistry. KPI- Impact factor of accepted journals, citations, author h-index. Course Materials, Conferences & Workshops: In June 2020, our partner ICTP (UNESCO flagship institute) will host Conference on the Complex Interactions of Light and Biological Matter: Experiments meet Theory. We will organize in a special AP session showcasing our project through posters and oral communications and will host a workshop and an information kiosk dedicated to SoFiA. A summer school for PhD students, on AP will be organized and hosted by UU (by M30) Our start-up executive body WI (non-beneficiary) is supported by Sofia Tech Park (STP) - a (Bulgarian flagship) EU project. With support of WI and STP we will host a workshop (by M46) on solar fuels with focus on AP in Bulgaria (energetically poor/unsustainable region), and tailored for an audience usually remote from the EU policy dialogue. All partners will attend the most relevant conferences (including MRS, ACS, ISF, etc.). SoFiA will also participate in the annual FET Conferences. Our IPR protected findings, concept design and selected experimental results will be included as graduate level course material at partner Universities. Course update plans will be included as chapters in final two project periodic reports on M30 & M48. KPI- Attendance in Summer School, Workshop, and attendee/student feedback. Related EU projects will be monitored and contacted. Key representatives will be invited for lectures at the Bulgaria workshop. SoFiA will enhance networking possibilities with the following programs: FET projects – A-Leaf (Proactive) and Diacat (Open), from ERC Grantees in AP (COFLeaf; ENLIGHT; HyMAP; HYMEM; photocatH2ode; TripleSolar; and others.) KPI- New collaborations for Phase II, III and feedback from AP experts. Dissemination to Industrial sector and to Policy Makers- SoFiA will participate in relevant industrial fairs, for instance: SSIS (smart systems industry summit), W3+FAIR. For critical coverage of breakthrough results we have identified policy journals: ENDS Europe, and Brussels based Politico and Euractiv. To communicate with EU policymakers, the coordinator will contact OBSERVE- a FET-CSA that supports Europe in FET, and FET2RIN, a network connecting FET projects to potential investors. Through EAB meetings, IPR protected research findings will be communicated to Shell, Air Liquide and Unilever who are interested in commercial exploitation. Climate & Policy experts at EAB will be consulted to indicate policy hook for market uptake. EAB feedback

Final update of Dissemination and Exploitation plan (si apre in una nuova finestra)
Project website with open and restricted access (si apre in una nuova finestra)

Project website & social media networking will be set up by M2 (D5.1) and updated on a monthly basis. We have a logo. Website will include news & events, links to partners’ websites, a press desk, publications, and search functionalities. The website will also promote important (public) results from related projects in AP and will administer an open forum as a knowledge-sharing tool for partners and user communities. Facebook, Twitter and LinkedIn will be used to promote the website content. An impact assessment of the entire social media communications activities will be carried out by monitoring web hits, likes, followers, retweets (KPI). Videos & news bytes will also be promoted through Hassim Al-Ghaili’s science communication website which has >16M fans. The existing Wikipedia page on AP will be updated with critical results from SoFiA.

Final update of Data management plan (si apre in una nuova finestra)
2nd update of Data management plan (si apre in una nuova finestra)
Data management plan (si apre in una nuova finestra)

Data management Plan (DMP): SoFiA will participate in the Pilot on Open Research Data and will provide open access to raw data corresponding to modelling & simulation, as well as data required to reproduce the results presented in scientific publications. These data will be stored in Zenodo (a research data repository created by CERN) ensuring their public availability and long-time preservation. Details will be provided in a data management plan (DMP, D6.3), to be delivered by M6 and updated periodically (M12, M30). Main modelling results will be disseminated through the European Materials Modelling Council ensuring wide research visibility. Publications: We will prioritise Gold or Green (with 6 months embargo) open access publication. At least 8 publications are estimated in journals with the highest impact in multidisciplinary science, in materials sciences, in nanotechnology, and in chemistry. KPI- Impact factor of accepted journals, citations, author h-index.

Pubblicazioni

Shorter Alkyl Chains Enhance Molecular Diffusion and Electron Transfer Kinetics between Photosensitisers and Catalysts in CO 2 -Reducing Photocatalytic Liposomes. (si apre in una nuova finestra)

Autori: David M. Klein; Santiago Rodríguez-Jiménez; Marlene E. Hoefnagel; Andrea Pannwitz; Andrea Pannwitz; Amrutha Prabhakaran; Maxime A. Siegler; Tia E. Keyes; Erwin Reisner; Albert M. Brouwer; Sylvestre Bonnet
Pubblicato in: Chem.Eur.J., Numero 2021, 27, 2021, Pagina/e 17203–17212, ISSN 0947-6539
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/chem.202102989

A novel concept of photosynthetic soft membranes: a numerical study (si apre in una nuova finestra)

Autori: Gabriele Falciani, Luca Bergamasco, Shannon A. Bonke, Indraneel Sen, Eliodoro Chiavazzo
Pubblicato in: Discover nano, 2023, Pagina/e 15, ISSN 2731-9229
Editore: Springer Nature
DOI: 10.1186/s11671-023-03772-1

Realizing Symmetry-Breaking Architectures in Soap Films (si apre in una nuova finestra)

Autori: Nidhi Kaul, Luca Bergamasco, Hongwei Song, Thijs Varkevisser, Agnese Amati, Gabriele Falciani, Cees J. M. van Rijn, Eliodoro Chiavazzo, Indraneel Sen, Sylvestre Bonnet, Leif Hammarström
Pubblicato in: Physical Review Letters, Numero 132, 2024, ISSN 0031-9007
Editore: American Physical Society
DOI: 10.1103/physrevlett.132.028201

Interfacial Characterization of Ruthenium-Based Amphiphilic Photosensitizers (si apre in una nuova finestra)

Autori: Yousra Timounay, Andrea Pannwitz, David M. Klein, Anne-Laure Biance, Marlene E. Hoefnagel, Indraneel Sen, Alain Cagna,* Marie Le Merrer,* and Sylvestre Bonnet*
Pubblicato in: Langmuir, Numero 38, 2022, 2022, Pagina/e 9697-9707, ISSN 0743-7463
Editore: American Chemical Society
DOI: 10.1021/acs.langmuir.2c01391

Water-Induced Restructuring of the Surface of a Deep Eutectic Solvent (si apre in una nuova finestra)

Autori: Rahul Gera, Carolyn J. Moll, Aditi Bhattacherjee, Huib J. Bakker
Pubblicato in: The Journal of Physical Chemistry Letters, Numero 13, 2023, Pagina/e 634-641, ISSN 1948-7185
Editore: American Chemical Society
DOI: 10.1021/acs.jpclett.1c03907

Multi-Variable Multi-Metric Optimisation of Self-Assembled Photocatalytic CO2 Reduction Performance using Machine Learning Algorithms (si apre in una nuova finestra)

Autori: Shannon Bonke, Giovanni Trezza, Luca Bergamasco, Hongwei Song, Santiago Rodríguez-Jiménez, Leif Hammarström, Eliodoro Chiavazzo, Erwin Reisner
Pubblicato in: Journal of the Americal Chemical Society, 2023, ISSN 0002-7863
Editore: American Chemical Society
DOI: 10.26434/chemrxiv-2023-g5hkm

Molecularly engineered photocatalyst sheet for scalable solar formate production from carbon dioxide and water (si apre in una nuova finestra)

Autori: Qian Wang, Julien Warnan, Santiago Rodríguez-Jiménez, Jane J. Leung, Shafeer Kalathil, Virgil Andrei, Kazunari Domen, Erwin Reisner
Pubblicato in: Nature Energy, 2020, ISSN 2058-7546
Editore: Nature
DOI: 10.1038/s41560-020-0678-6

Observation of Strong Synergy in the Interfacial Water Response of Binary Ionic and Nonionic Surfactant Mixtures (si apre in una nuova finestra)

Autori: Sanghamitra Sengupta, Rahul Gera, Colin Egan, Uriel N. Morzan, Jan Versluis, Ali Hassanali, Huib J. Bakker
Pubblicato in: The Journal of Physical Chemistry Letters, Numero 13, 2023, Pagina/e 11391-11397, ISSN 1948-7185
Editore: American Chemical Society
DOI: 10.1021/acs.jpclett.2c02750

Mechanistic Insights into the Charge Transfer Dynamics of Photocatalytic Water Oxidation at the Lipid Bilayer−Water Interface (si apre in una nuova finestra)

Autori: Hongwei Song, Agnese Amati, Andrea Pannwitz, Sylvestre Bonnet, and Leif Hammarström
Pubblicato in: The Journal of the American Chemical Society, Numero 144, 2022, 2022, Pagina/e 19353−19364, ISSN 0002-7863
Editore: American Chemical Society
DOI: 10.1021/jacs.2c06842

Emergence of Electric Fields at the Water–C12E6 Surfactant Interface (si apre in una nuova finestra)

Autori: Rahul Gera, Huib J. Bakker, Ricardo Franklin-Mergarejo, Uriel N. Morzan, Gabriele Falciani, Luca Bergamasco, Jan Versluis, Indraneel Sen, Silvia Dante, Eliodoro Chiavazzo, and Ali A. Hassanali
Pubblicato in: J. Am. Chem. Soc., Numero 2021, 143, 37, 2021, Pagina/e 15103–15112, ISSN 0002-7863
Editore: American Chemical Society
DOI: 10.26434/chemrxiv.14661360.v1

Roadmap towards solar fuel synthesis at the water interface of liposome membranes (si apre in una nuova finestra)

Autori: A. Pannwitz, D.M. Klein, S. Rodríguez-Jiménez, C. Casadevall, H. Song, E. Reisner, L. Hammarström, S. Bonnet
Pubblicato in: Chem. Soc. Rev.,, Numero 50, 2021, 2021, Pagina/e 4833–4855, ISSN 0306-0012
Editore: Royal Society of Chemistry
DOI: 10.1039/d0cs00737d

An overview on modelling approaches for photochemical and photoelectrochemical solar fuels processes and technologies (si apre in una nuova finestra)

Autori: Gabriele Falciani, Eliodoro Chiavazzo
Pubblicato in: Energy Conversion and Management, 2023, ISSN 0196-8904
Editore: Pergamon Press Ltd.
DOI: 10.1016/j.enconman.2023.117366

Self-Assembled Liposomes Enhance Electron Transfer for Efficient Photocatalytic CO2 Reduction (si apre in una nuova finestra)

Autori: "Santiago Rodríguez-Jiménez,# Hongwei Song,# Erwin Lam, Demelza Wright, Andrea Pannwitz, Shannon A. Bonke, Jeremy J. Baumberg, Sylvestre Bonnet, Leif Hammarström,* and Erwin Reisner*"
Pubblicato in: The Journal of the American Chemical Society, Numero 144, 2022, 2022, Pagina/e 9399−9412, ISSN 0002-7863
Editore: American Chemical Society
DOI: 10.1021/jacs.2c01725

Free energy decompositions illuminate synergistic effects in interfacial binding thermodynamics of mixed surfactant systems (si apre in una nuova finestra)

Autori: Colin K. Egan, Ali Hassanali
Pubblicato in: The Journal of Chemical Physics, Numero 159, 2023, ISSN 0021-9606
Editore: American Institute of Physics
DOI: 10.1063/5.0163849

Design and testing of a device for the characterization of gas transfer through soap films and measurement protocol based on color matching (si apre in una nuova finestra)

Autori: Gabriele Falciani, Luca Bergamasco, Agnese Amati, Gijsbert Verdoes, Indraneel Sen, Sylvestre Bonnet, Eliodoro Chiavazzo
Pubblicato in: International Communications in Heat and Mass Transfer, Numero 149, 2023, Pagina/e 107161, ISSN 0735-1933
Editore: Pergamon Press Ltd.
DOI: 10.1016/j.icheatmasstransfer.2023.107161

A multi-scale perspective of gas transport through soap-film membranes (si apre in una nuova finestra)

Autori: Gabriele Falciani, Ricardo Franklin, Alain Cagna, Indraneel Sen, Ali Hassanali, Eliodoro Chiavazzo
Pubblicato in: Molecular Systems Design & Engineering, Numero 5/5, 2020, Pagina/e 911-921, ISSN 2058-9689
Editore: Royal Society of Chemistry
DOI: 10.1039/c9me00186g

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