GEN IV Integrated Oxide fuels recycling strategies

CORDIS proporciona enlaces a los documentos públicos y las publicaciones de los proyectos de los programas marco HORIZONTE.

Los enlaces a los documentos y las publicaciones de los proyectos del Séptimo Programa Marco, así como los enlaces a algunos tipos de resultados específicos, como conjuntos de datos y «software», se obtienen dinámicamente de OpenAIRE .

Resultado final

Status on the PyTri-Diol properties

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Communication and dissemination action plan

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"Impact of the precursor ""history"" (nature, structural, microstructural and morphological parameters) during the conversion and sintering to actinide based dioxide materials"

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Destruction of organic

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WPASR 6

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Innovative dissolution routes for highly plutonium doped (U,Pu)O2 and (U,Pu,MA)O2 samples

Old number D142

Clustering Events 1

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Impact assessment report for fuel cycle implications

Old number D315

Clustering Events 3

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Product quality, characterization & testing

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Status on TODGA organic phase loading

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report on travel bursary and secondment grant attribution

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WPASR 1

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Performances on microelectrode for online monitoring of relevant parameters

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Draft iSanex/Ganex package ready for testing

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Impacts on process safety of gas generation

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Major Hazard and Criticality review of the Euro-Ganex process

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contribution of computational multi-disciplinary approaches to the design of solvent extraction devices

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Knowledge and Data Management Plan

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optimized flowsheets for homogeneous recycling of advanced MOX fuel in GEN IV reactors

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Status on solvent clean-up & recycling

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Molecular modeling of particular degradation mechanism of extracting and complexing agents

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WPASR 2

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Report on the development of the different MABB precursor synthesis routes and their contribution on MA homogeneity, dust reduction, lowering sintering temperature

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Report with collected data on the main solvents and the density laws build

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WPASR 4

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Report on dissolution model development

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Mapping of the different status and alternatives for each ESNII concept

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organisation of the think-tank event

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Stability and safety studies of hold extraction systems (1 for each CyMe4BTBP, HidroBTBP, TODGA & PTD)

Old number D121

Assessment of applications of PTD in i-SANEX and EUROGANEX processes

Old number D221

Report on the methodology to establish a density law for NCS evaluations. It will include the needs in terms of data and chemical measurements

Old number D323

WPASR 5

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Report on hazard analysis mainly focusing on criticality aspects

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Packages tested and released

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Experimental and modeling studies of transfer kinetics in the reference separation processes

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Report on the comparison of SX processes for heterogeneous recycling

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optimized flowsheets for heterogeneous recycling of advanced MOX fuel in GEN IV reactors

Old number D223

Report on efficiency of the electrochemical decomposition of ligands from SX processes and on its inputs on MABB precursor properties

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Status on Distribution data and chemical modelling

Old number D132

Project website

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Clustering Events 4

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Communication toolkit

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Identification of optimized conditions for effecter fission product masking/scrubbing

Old number D112

Clustering Events 2

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Safety Review minutes, including recommendations for future R&D which could eliminate, reduce or mitigate hazards

Old number D312

Report on the speciation and extraction of key fission products

Old number D111

WPASR 3

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Understanding the evolution of an interface during dissolution of actinide oxide materials by macro/microscopic approaches combination

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Assessment of the corrosion vulnerability of common plant materials in the presence of key process streams

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studies of non-powder routes for the synthesis of MOX fuels materials, potentially bearing minor actinides and blanket fuel materials

Old number D143

deliverable report on specification for on line packages

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Stability studies of stripping agents

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Process Description report of Concept Euro-GANEX Plant

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Report on ‘Sim-Plant’ Methodology and flowsheet comparison

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WPASR 7

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Status of flowsheet calculations made for WP22 process testing

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Draft Purex package ready for testing

Old number D424

Impacts of solvent degradation and recycle on the EURO-GANEX process

Old number D212

Stakeholders Event 2

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Exploitation plan based on the conclusions of the interactions with stakeholders/end-users

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Stakeholders Event 1

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Publicaciones

Characteristics of the extraction systems for the minor actinoids and lanthanoids separation using hydrophilic masking agents and TODGA

Autores: Šebesta, J.; Distler, P.; John, J.; Bavol, D.; Gruner, B.
Publicado en: Czech Chemical Society Symposium Series, Edición Volume 18, issue 3, 2020, 2020, Página(s) 157-158, ISSN 2336-7210
Editor: Česká společnost chemická

Study of the effect of radiation on the Ln (III)/An(III) separation in the systems using hydrophilic masking agents during extraction into TODGA

Autores: Šebesta, J.; Distler, P.; John, J.
Publicado en: Jaderná energetika v pracích mladé generace 2019., Edición 2020, 2020, Página(s) 128-133, ISBN 978-80-02-02895-6
Editor: Česká nukleární společnost

Characterization of Am(III) and Eu(III) extraction in the CHALMEX systems

Autores: Mindová, M.; Distler, P.; John, J.; Bavol, D.; Gruner, B.
Publicado en: Czech Chemical Society Symposium Series, Edición Volume 18, Edición 3, 2020, 2020, Página(s) 157, ISSN 2336-7210
Editor: Česká společnost chemická

Attempts to isolate technetium in the process of separating actinides from spent nuclear fuel (in Polish)

Autores: Magdalena Rejnis-Strzelak, Irena Herdzik-Koniecko, Jerzy Narbutt
Publicado en: Abstracts, 62nd Annual Scientific Meeting of the Polish Chemical Society, Warsaw, Sep. 2-6, 2019, Edición Poster S16 P10, 2019, Página(s) page S16-25
Editor: Polish Chemical Society

Influence of gamma radiation on the properties of Ln(III)/An(III) extractiion systems using the lipophilic extractant CyMe4-BTBP

Autores: Mindová, M.; Distler, P.
Publicado en: Jaderná energetika v pracích mladé generace 2019, Edición 2020, 2020, Página(s) 123-127, ISBN 978-80-02-02895-6
Editor: Česká nukleární společnost

Solvent extraction of americium from spent nuclear fuel and closing the fuel cycle - new perspectives for development of nuclear energy (in Polish)

Autores: Jerzy Narbutt
Publicado en: Abstracts, 62nd Annual Scientific Meeting of the Polish Chemical Society, Warsaw, Sep. 2-6, 2019, Edición Section lecture S16 WS03, 2019, Página(s) page S16-6
Editor: Polish Chemical Society

A review of ageing, hydrolysis and radiolysis effects on PyTri-based stripping solvents for i-SANEX/GANEX processes

Autores: E. Mossini, E. Macerata, M.C. Charbonnel, A. Casnati, A. Mele, A. Geist, M. Mariani
Publicado en: RB2018 - Second edition of Radical Behaviour workshop, 2018
Editor: E. Mossini

FLUORINATED CARBONATES AS NEW DILUENTS FOR EXTRACTION OF F-ELEMENTS

Autores: VASILIY BABAIN, MIKHAIL ALYAPYSHEV, I.G. VORONAEV, LIUDMILA TKACHENKO, E.V. KENF, MIRIAM MINDOVÁ, PETR DISTLER, JAN JOHN
Publicado en: Czech Chemical Society Symposium Series, Edición Vol. 16, No. 2, 2018, Página(s) p. 135, ISSN 2336-7202
Editor: Czech Chemical Society

APPLICATION OF MOLECULAR MODELLING FOR STUDYING THE STABILITY OF ORGANIC LIGANDS IN NUCLEAR FUEL CYCLE

Autores: TOMÁŠ KOUBSKÝ, LADISLAV KALVODA
Publicado en: Czech Chemical Society Symposium Series, Edición Vol. 16, No. 2, 2018, Página(s) p. 81, ISSN 2336-7202
Editor: Czech Chemical Society

PARTITIONING OF MINOR AN(III) AND LN(III) BY THE 1,2,4-TRIAZINE EXTRACTING COMPOUNDS

Autores: PETR DISTLER, ASHFAQ AFSAR, KAMILA ŠŤASTNÁ, JAMES WESTWOOD, FRANK W. LEWIS, KAREL ŠTAMBERG, LAURENCE HARWOOD, JAN JOHN
Publicado en: Czech Chemical Society Symposium Series, Edición Vol. 16, No. 2, 2018, Página(s) p. 56, ISSN 2336-7202
Editor: Czech Chemical Society

Problem of a Thorough Geometric Optimization

Autores: Tomáš Koubský
Publicado en: Proceedings of the 7th students´ science conference on the solid state physics and materials, Edición 2017-09-18 / 2017-09-22, 2018, Página(s) p. 20-22, ISBN 978-80-01-06374-3
Editor: Czech Technical University Publishing House

Study of organic ligands by classical simulation methods (in Czech: Studium organických ligandů klasickými simulačními metodami)

Autores: Lucie Celbová
Publicado en: Proceedings of the 8th students´ science conference on the solid state physics and materials, Edición Sedliště, 17-21/09/2018, 2018, Página(s) pp. 11-13, ISBN 978-80-01-06511-2
Editor: CTU in Prague

Fluorinated Carbonates as New Diluents for Extraction of f-Elements

Autores: Babain, V.A.; Alyapyshev, M.Yu.; Voronaev, I.G.; Tkachenko, L.I.; Kenf, E.V.; Mindová, M.; Distler, P.; John, J.
Publicado en: Czech Chemical Society, Symposium Series, Edición Volume 16, Edición 2, 2018, 2018, Página(s) 135, ISSN 2336-7202
Editor: Česká společnost chemická

Optimizing the separation of fission product technetium in the process of recycling actinides from spent nuclear fuel

Autores: Irena Herdzik-Koniecko, Magdalena Rejnis-Strzelak, Jerzy Narbutt
Publicado en: International Conference on Development and Applications of Nuclear Technologies, NUTECH-2020, Conference Abstracts, Edición Poster, Warsaw, 4-7 October 2020, 2020, Página(s) Conference Abstracts & Programme, page 56, ISBN 978-83-946412-4-5
Editor: Institute of Nuclear Chemistry and Technology

Fluorinated Carbonates as New Diluents for Extraction and Separation of f- Block Elements

Autores: Petr Distler, Miriam Mindová, Jan John, Vasilij A. Babain, Mikhail Yu. Alyapyshev, Lyudmila I. Tkachenko, Ekaterina V. Kenf, Laurence M. Harwood, Ashfaq Afsar
Publicado en: Solvent Extraction and Ion Exchange, Edición 38/2, 2020, Página(s) 180-193, ISSN 0736-6299
Editor: Marcel Dekker Inc.
DOI: 10.1080/07366299.2019.1708004

Stability of Different BTBP and BTPhen Extracting or Masking Compounds Against Gamma Radiation

Autores: Distler P., Mindova M., Šebesta J., Grűner B., Bavol D., Egberink R. J. M., Verboom W., Babain V. A., John J.,
Publicado en: Chemistry Research, Edición 24 issues/ year, 2021, Página(s) 19 MS pages, ISSN 1520-5045
Editor: American Chemical Society

The conversion of ammonium uranate prepared via sol-gel synthesis into uranium oxides

Autores: Christian Schreinemachers, Gregory Leinders, Giuseppe Modolo, Marc Verwerft, Koen Binnemans, Thomas Cardinaels
Publicado en: Nuclear Engineering and Technology, Edición 52/5, 2020, Página(s) 1013-1021, ISSN 1738-5733
Editor: Korean Nuclear Society
DOI: 10.1016/j.net.2019.11.004

Separation of Minor Actinides from Lanthanides Using Immobilized Ligand Systems: The Role of the Counterion

Autores: Laurence M. Harwood, Ashfaq Afsar, Petr Distler, Jan John, Jasraj S. Babra, Zoe Y. Selfe, Joeseph Cowell, James Westwood
Publicado en: HETEROCYCLES, Edición 99/2, 2019, Página(s) 825, ISSN 0385-5414
Editor: Elsevier BV
DOI: 10.3987/com-18-s(f)71

Structural changes of Nd- and Ce-doped ammonium diuranate microspheres during the conversion to U1−LnO2±

Autores: Christian Schreinemachers, Gregory Leinders, Renaud Podor, Joseph Lautru, Nicolas Clavier, Giuseppe Modolo, Marc Verwerft, Koen Binnemans, Thomas Cardinaels
Publicado en: Journal of Nuclear Materials, Edición 542, 2020, Página(s) 152454, ISSN 0022-3115
Editor: Elsevier BV
DOI: 10.1016/j.jnucmat.2020.152454

Solvent Extraction Investigations on Pu(IV) and Th(IV) Complexes with Hydrophilic SO 3 -Ph-BTP and SO 3 -Ph-BTBP Ligands

Autores: Łukasz Steczek, Jerzy Narbutt, Marie-Christine Charbonnel, Philippe Moisy
Publicado en: Solvent Extraction and Ion Exchange, Edición 37/3-4, 2019, Página(s) 259-268, ISSN 0736-6299
Editor: Marcel Dekker Inc.
DOI: 10.1080/07366299.2019.1639366

A Study of Cerium Extraction Kinetics by TODGA in Acidified and Non-Acidified Organic Solvent Phases in the Context of Fission Product Management

Autores: Michael Anthony Bromley Colin Boxall
Publicado en: Progress in Nuclear Science and Technology, 2018, Página(s) 70-73, ISSN 2185-4823
Editor: Atomic Energy Society of Japan
DOI: 10.15669/pnst.5.70

On the Basic Extraction Properties of a Phenyl Trifluoromethyl Sulfone-Based GANEX System Containing CyMe 4 -BTBP and TBP

Autores: Jenny Halleröd, Christian Ekberg, Thea Authen, Laura Bertolo, Mu Lin, Bohumír Grüner, Jaroslav Švehla, Christoph Wagner, Andreas Geist, Petra Panak, Emma Aneheim
Publicado en: Solvent Extraction and Ion Exchange, Edición 36/4, 2018, Página(s) 360-372, ISSN 0736-6299
Editor: Marcel Dekker Inc.
DOI: 10.1080/07366299.2018.1497043

Radiolytic and hydrolytic degradation of the hydrophilic diglycolamides

Autores: Andreas Wilden, Bruce J. Mincher, Stephen P. Mezyk, Liam Twight, Kristyn M. Rosciolo-Johnson, Christopher A. Zarzana, Mary E. Case, Michelle Hupert, Andrea Stärk, Giuseppe Modolo
Publicado en: Solvent Extraction and Ion Exchange, Edición 36/4, 2018, Página(s) 347-359, ISSN 0736-6299
Editor: Marcel Dekker Inc.
DOI: 10.1080/07366299.2018.1495384

Stoichiometry of An( iii )–DMDOHEMA complexes formed during solvent extraction

Autores: Patrik Weßling, Michael Trumm, Andreas Geist, Petra J. Panak
Publicado en: Dalton Transactions, Edición 47/32, 2018, Página(s) 10906-10914, ISSN 1477-9226
Editor: Royal Society of Chemistry
DOI: 10.1039/c8dt02504e

Modified diglycolamides for grouped actinide separation

Autores: Rikard Malmbeck, Daniel Magnusson, Andreas Geist
Publicado en: Journal of Radioanalytical and Nuclear Chemistry, Edición 314/3, 2017, Página(s) 2531-2538, ISSN 0236-5731
Editor: Akademiai Kiado
DOI: 10.1007/s10967-017-5614-2

Optimization and Single-Stage Centrifugal Contactor Experiments with the Novel Hydrophilic Complexant PyTri-Diol for the i -SANEX Process

Autores: Eros Mossini, Elena Macerata, Andreas Wilden, Peter Kaufholz, Giuseppe Modolo, Nicolò Iotti, Alessandro Casnati, Andreas Geist, Mario Mariani
Publicado en: Solvent Extraction and Ion Exchange, Edición 36/4, 2018, Página(s) 373-386, ISSN 0736-6299
Editor: Marcel Dekker Inc.
DOI: 10.1080/07366299.2018.1507134

Behaviour of the extractant Me-TODGA upon gamma irradiation: quantification of degradation compounds and individual influences on complexation and extraction

Autores: V. Hubscher-Bruder, V. Mogilireddy, S. Michel, A. Leoncini, J. Huskens, W. Verboom, H. Galán, A. Núñez, J. Cobos, G. Modolo, A. Wilden, H. Schmidt, M.-C. Charbonnel, P. Guilbaud, N. Boubals
Publicado en: New Journal of Chemistry, Edición 41/22, 2017, Página(s) 13700-13711, ISSN 1144-0546
Editor: Royal Society of Chemistry
DOI: 10.1039/c7nj02136d

Synthesis of size-controlled UO 2 microspheres from the hydrothermal conversion of U( iv ) aspartate

Autores: V. Trillaud, J. Maynadié, J. Manaud, J. Hidalgo, D. Meyer, R. Podor, N. Dacheux, N. Clavier
Publicado en: CrystEngComm, Edición 20/48, 2018, Página(s) 7749-7760, ISSN 1466-8033
Editor: Royal Society of Chemistry
DOI: 10.1039/c8ce01352g

2,6-Bis(1-alkyl-1H-1,2,3-triazol-4-yl)-pyridines: selective lipophilic chelating ligands for minor actinides

Autores: Annalisa Ossola, Elena Macerata, Eros Mossini, Marco Giola, Maria Chiara Gullo, Arturo Arduini, Alessandro Casnati, Mario Mariani
Publicado en: Journal of Radioanalytical and Nuclear Chemistry, Edición 318/3, 2018, Página(s) 2013-2022, ISSN 0236-5731
Editor: Akademiai Kiado
DOI: 10.1007/s10967-018-6253-y

Application of quantum mechanical simulations for studying the radiolytic stability of prospective extractants in the nuclear fuel cycle

Autores: Tomáš Koubský, Jakub Luštinec
Publicado en: Journal of Radioanalytical and Nuclear Chemistry, Edición 318/3, 2018, Página(s) 2407-2413, ISSN 0236-5731
Editor: Akademiai Kiado
DOI: 10.1007/s10967-018-6225-2

Extraction Properties of 4-Tetra(hydroxyphenyl)BTPhen in Liquid-Liquid Extraction Systems with Cyclohexanone/Octanol or in a Solid-Phase Extraction System

Autores: Laurence M. Harwood, Jan John, Ashfaq Afsar, Jasraj S. Babra, Petr Distler, Iain Hopkins, James Westwood, Zoe Y. Selfe
Publicado en: HETEROCYCLES, Edición 101/1, 2020, Página(s) 209, ISSN 0385-5414
Editor: Elsevier BV
DOI: 10.3987/com-19-s(f)14

Thermodynamic parameters of Am(III), Cm(III) and Eu(III) extraction by CyMe4-BTPhen in cyclohexanone from HNO3 solutions

Autores: Petr Distler, Karel Stamberg, Jan John, Laurence M. Harwood, Frank W. Lewis
Publicado en: The Journal of Chemical Thermodynamics, Edición 141, 2020, Página(s) 105955, ISSN 0021-9614
Editor: Academic Press
DOI: 10.1016/j.jct.2019.105955

Activation of the Aromatic Core of 3,3′-(Pyridine-2,6-diylbis(1 H -1,2,3-triazole-4,1-diyl))bis(propan-1-ol)—Effects on Extraction Performance, Stability Constants, and Basicity

Autores: Patrik Weßling, Michael Trumm, Elena Macerata, Annalisa Ossola, Eros Mossini, Maria Chiara Gullo, Arturo Arduini, Alessandro Casnati, Mario Mariani, Christian Adam, Andreas Geist, Petra J. Panak
Publicado en: Inorganic Chemistry, Edición 58/21, 2019, Página(s) 14642-14651, ISSN 0020-1669
Editor: American Chemical Society
DOI: 10.1021/acs.inorgchem.9b02325

On the basic extraction properties of a phenyl trifuoromethyl sulfone based GANEX system containing CyMe4-BTBP and TBP.

Autores: J. Halleröd, Ch. Ekberg, T. Authen, L. Bertolo, Mu Lin, B. Grüner, J. Švehla, Ch. Wagner, A. Geist, P. Panak, E. Aneheim.
Publicado en: Solvent Extraction and Ion Exchange, Edición Vol. 36, Edición 4, 2018, Página(s) 360-372, ISSN 0736-6299
Editor: Marcel Dekker Inc.
DOI: 10.1080/07366299.2018.1497043

Stability studies of GANEX system under different irradiation conditions

Autores: Iván Sánchez-García, Hitos Galán, Jose Manuel Perlado, Joaquín Cobos
Publicado en: EPJ Nuclear Sciences & Technologies, Edición 5, 2019, Página(s) 19, ISSN 2491-9292
Editor: EDP Sciences
DOI: 10.1051/epjn/2019049

Do An( iii ) and Ln( iii ) ions form heteroleptic complexes with diglycolamide and hydrophilic BT(B)P ligands in solvent extraction systems? A spectroscopic and DFT study

Autores: Irena Herdzik-Koniecko, Christoph Wagner, Michael Trumm, Udo Müllich, Bernd Schimmelpfennig, Jerzy Narbutt, Andreas Geist, Petra J. Panak
Publicado en: New Journal of Chemistry, Edición 43/16, 2019, Página(s) 6314-6322, ISSN 1144-0546
Editor: Royal Society of Chemistry
DOI: 10.1039/c9nj00651f

Gamma and pulsed electron radiolysis studies of CyMe4BTBP and CyMe4BTPhen: identification of radiolysis products and effects on the hydrometallurgical separation of trivalent actinides and lanthanides

Autores: Schmidt H., Wilden* A., Modolo G., Bosbach D., Santiago-Schübel B., HupertM., Mincher B. J., Mezyk S. P., Švehla J., Grüner B., Ekberg Ch.,
Publicado en: Radiation Phys. Chem., Edición 12 issues/ year, 2021, Página(s) 31 pp., ISSN 0969-806X
Editor: Pergamon Press Ltd.

Evaluation of the Hydrophilic Complexant N,N,N’,N’ -tetraethyldiglycolamide (TEDGA) and its Methyl-substituted Analogues in the Selective Am(III) Separation

Autores: Larissa Klaß, Andreas Wilden, Fabian Kreft, Christoph Wagner, Andreas Geist, Petra J. Panak, Irena Herdzik-Koniecko, Jerzy Narbutt, Giuseppe Modolo
Publicado en: Solvent Extraction and Ion Exchange, Edición 37/5, 2019, Página(s) 297-312, ISSN 0736-6299
Editor: Marcel Dekker Inc.
DOI: 10.1080/07366299.2019.1651039

Fabrication of Nd- and Ce-doped uranium dioxide microspheres via internal gelation

Autores: Christian Schreinemachers; Gregory Leinders; Giuseppe Modolo; Marc Verwerft; Koen Binnemans; Thomas Cardinaels
Publicado en: Journal of Nuclear Materials, Edición 21, 2020, ISSN 0022-3115
Editor: Elsevier BV

Solvent Extraction for Nuclear Power

Autores: Jerzy Narbutt
Publicado en: Liquid-Phase Extraction, Edición Handbooks in Separation Science, Colin F. Poole, Editor, 2020, Página(s) 725-744, ISBN 9780128169117
Editor: Elsevier
DOI: 10.1016/b978-0-12-816911-7.00024-4

The use of synergistic effects of lipophilic modifiers of TODGA-containing organic phase for improving separation of Am(III) from the early lanthanides in the process of stripping the metals with hydrophilic ligands. A novel concept for solving the problem

Autores: Jerzy Narbutt, Irena Herdzik-Koniecko, Magdalena Rejnis-Strzelak
Publicado en: RAPORTY IChTJ, SERIA B, Edición Nr 2/2017, 2017, Página(s) 1 - 14, ISSN 1425-7351
Editor: ICHTJ

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