GEN IV Integrated Oxide fuels recycling strategies

CORDIS fornisce collegamenti ai risultati finali pubblici e alle pubblicazioni dei progetti ORIZZONTE.

I link ai risultati e alle pubblicazioni dei progetti del 7° PQ, così come i link ad alcuni tipi di risultati specifici come dataset e software, sono recuperati dinamicamente da .OpenAIRE .

Risultati finali

Status on the PyTri-Diol properties

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Communication and dissemination action plan

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"Impact of the precursor ""history"" (nature, structural, microstructural and morphological parameters) during the conversion and sintering to actinide based dioxide materials"

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Destruction of organic

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WPASR 6

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Innovative dissolution routes for highly plutonium doped (U,Pu)O2 and (U,Pu,MA)O2 samples

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Clustering Events 1

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Impact assessment report for fuel cycle implications

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Clustering Events 3

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Product quality, characterization & testing

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Status on TODGA organic phase loading

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report on travel bursary and secondment grant attribution

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WPASR 1

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Performances on microelectrode for online monitoring of relevant parameters

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Draft iSanex/Ganex package ready for testing

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Impacts on process safety of gas generation

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Major Hazard and Criticality review of the Euro-Ganex process

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contribution of computational multi-disciplinary approaches to the design of solvent extraction devices

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Knowledge and Data Management Plan

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optimized flowsheets for homogeneous recycling of advanced MOX fuel in GEN IV reactors

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Status on solvent clean-up & recycling

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Molecular modeling of particular degradation mechanism of extracting and complexing agents

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WPASR 2

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Report on the development of the different MABB precursor synthesis routes and their contribution on MA homogeneity, dust reduction, lowering sintering temperature

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Report with collected data on the main solvents and the density laws build

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WPASR 4

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Report on dissolution model development

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Mapping of the different status and alternatives for each ESNII concept

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organisation of the think-tank event

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Stability and safety studies of hold extraction systems (1 for each CyMe4BTBP, HidroBTBP, TODGA & PTD)

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Assessment of applications of PTD in i-SANEX and EUROGANEX processes

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Report on the methodology to establish a density law for NCS evaluations. It will include the needs in terms of data and chemical measurements

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WPASR 5

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Report on hazard analysis mainly focusing on criticality aspects

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Packages tested and released

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Experimental and modeling studies of transfer kinetics in the reference separation processes

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Report on the comparison of SX processes for heterogeneous recycling

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optimized flowsheets for heterogeneous recycling of advanced MOX fuel in GEN IV reactors

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Report on efficiency of the electrochemical decomposition of ligands from SX processes and on its inputs on MABB precursor properties

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Status on Distribution data and chemical modelling

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Project website

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Clustering Events 4

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Communication toolkit

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Identification of optimized conditions for effecter fission product masking/scrubbing

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Clustering Events 2

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Safety Review minutes, including recommendations for future R&D which could eliminate, reduce or mitigate hazards

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Report on the speciation and extraction of key fission products

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WPASR 3

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Understanding the evolution of an interface during dissolution of actinide oxide materials by macro/microscopic approaches combination

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Assessment of the corrosion vulnerability of common plant materials in the presence of key process streams

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studies of non-powder routes for the synthesis of MOX fuels materials, potentially bearing minor actinides and blanket fuel materials

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deliverable report on specification for on line packages

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Stability studies of stripping agents

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Process Description report of Concept Euro-GANEX Plant

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Report on ‘Sim-Plant’ Methodology and flowsheet comparison

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WPASR 7

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Status of flowsheet calculations made for WP22 process testing

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Draft Purex package ready for testing

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Impacts of solvent degradation and recycle on the EURO-GANEX process

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Stakeholders Event 2

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Exploitation plan based on the conclusions of the interactions with stakeholders/end-users

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Stakeholders Event 1

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Pubblicazioni

Characteristics of the extraction systems for the minor actinoids and lanthanoids separation using hydrophilic masking agents and TODGA

Autori: Šebesta, J.; Distler, P.; John, J.; Bavol, D.; Gruner, B.
Pubblicato in: Czech Chemical Society Symposium Series, Numero Volume 18, issue 3, 2020, 2020, Pagina/e 157-158, ISSN 2336-7210
Editore: Česká společnost chemická

Study of the effect of radiation on the Ln (III)/An(III) separation in the systems using hydrophilic masking agents during extraction into TODGA

Autori: Šebesta, J.; Distler, P.; John, J.
Pubblicato in: Jaderná energetika v pracích mladé generace 2019., Numero 2020, 2020, Pagina/e 128-133, ISBN 978-80-02-02895-6
Editore: Česká nukleární společnost

Characterization of Am(III) and Eu(III) extraction in the CHALMEX systems

Autori: Mindová, M.; Distler, P.; John, J.; Bavol, D.; Gruner, B.
Pubblicato in: Czech Chemical Society Symposium Series, Numero Volume 18, Numero 3, 2020, 2020, Pagina/e 157, ISSN 2336-7210
Editore: Česká společnost chemická

Attempts to isolate technetium in the process of separating actinides from spent nuclear fuel (in Polish)

Autori: Magdalena Rejnis-Strzelak, Irena Herdzik-Koniecko, Jerzy Narbutt
Pubblicato in: Abstracts, 62nd Annual Scientific Meeting of the Polish Chemical Society, Warsaw, Sep. 2-6, 2019, Numero Poster S16 P10, 2019, Pagina/e page S16-25
Editore: Polish Chemical Society

Influence of gamma radiation on the properties of Ln(III)/An(III) extractiion systems using the lipophilic extractant CyMe4-BTBP

Autori: Mindová, M.; Distler, P.
Pubblicato in: Jaderná energetika v pracích mladé generace 2019, Numero 2020, 2020, Pagina/e 123-127, ISBN 978-80-02-02895-6
Editore: Česká nukleární společnost

Solvent extraction of americium from spent nuclear fuel and closing the fuel cycle - new perspectives for development of nuclear energy (in Polish)

Autori: Jerzy Narbutt
Pubblicato in: Abstracts, 62nd Annual Scientific Meeting of the Polish Chemical Society, Warsaw, Sep. 2-6, 2019, Numero Section lecture S16 WS03, 2019, Pagina/e page S16-6
Editore: Polish Chemical Society

A review of ageing, hydrolysis and radiolysis effects on PyTri-based stripping solvents for i-SANEX/GANEX processes

Autori: E. Mossini, E. Macerata, M.C. Charbonnel, A. Casnati, A. Mele, A. Geist, M. Mariani
Pubblicato in: RB2018 - Second edition of Radical Behaviour workshop, 2018
Editore: E. Mossini

FLUORINATED CARBONATES AS NEW DILUENTS FOR EXTRACTION OF F-ELEMENTS

Autori: VASILIY BABAIN, MIKHAIL ALYAPYSHEV, I.G. VORONAEV, LIUDMILA TKACHENKO, E.V. KENF, MIRIAM MINDOVÁ, PETR DISTLER, JAN JOHN
Pubblicato in: Czech Chemical Society Symposium Series, Numero Vol. 16, No. 2, 2018, Pagina/e p. 135, ISSN 2336-7202
Editore: Czech Chemical Society

APPLICATION OF MOLECULAR MODELLING FOR STUDYING THE STABILITY OF ORGANIC LIGANDS IN NUCLEAR FUEL CYCLE

Autori: TOMÁŠ KOUBSKÝ, LADISLAV KALVODA
Pubblicato in: Czech Chemical Society Symposium Series, Numero Vol. 16, No. 2, 2018, Pagina/e p. 81, ISSN 2336-7202
Editore: Czech Chemical Society

PARTITIONING OF MINOR AN(III) AND LN(III) BY THE 1,2,4-TRIAZINE EXTRACTING COMPOUNDS

Autori: PETR DISTLER, ASHFAQ AFSAR, KAMILA ŠŤASTNÁ, JAMES WESTWOOD, FRANK W. LEWIS, KAREL ŠTAMBERG, LAURENCE HARWOOD, JAN JOHN
Pubblicato in: Czech Chemical Society Symposium Series, Numero Vol. 16, No. 2, 2018, Pagina/e p. 56, ISSN 2336-7202
Editore: Czech Chemical Society

Problem of a Thorough Geometric Optimization

Autori: Tomáš Koubský
Pubblicato in: Proceedings of the 7th students´ science conference on the solid state physics and materials, Numero 2017-09-18 / 2017-09-22, 2018, Pagina/e p. 20-22, ISBN 978-80-01-06374-3
Editore: Czech Technical University Publishing House

Study of organic ligands by classical simulation methods (in Czech: Studium organických ligandů klasickými simulačními metodami)

Autori: Lucie Celbová
Pubblicato in: Proceedings of the 8th students´ science conference on the solid state physics and materials, Numero Sedliště, 17-21/09/2018, 2018, Pagina/e pp. 11-13, ISBN 978-80-01-06511-2
Editore: CTU in Prague

Fluorinated Carbonates as New Diluents for Extraction of f-Elements

Autori: Babain, V.A.; Alyapyshev, M.Yu.; Voronaev, I.G.; Tkachenko, L.I.; Kenf, E.V.; Mindová, M.; Distler, P.; John, J.
Pubblicato in: Czech Chemical Society, Symposium Series, Numero Volume 16, Numero 2, 2018, 2018, Pagina/e 135, ISSN 2336-7202
Editore: Česká společnost chemická

Optimizing the separation of fission product technetium in the process of recycling actinides from spent nuclear fuel

Autori: Irena Herdzik-Koniecko, Magdalena Rejnis-Strzelak, Jerzy Narbutt
Pubblicato in: International Conference on Development and Applications of Nuclear Technologies, NUTECH-2020, Conference Abstracts, Numero Poster, Warsaw, 4-7 October 2020, 2020, Pagina/e Conference Abstracts & Programme, page 56, ISBN 978-83-946412-4-5
Editore: Institute of Nuclear Chemistry and Technology

Fluorinated Carbonates as New Diluents for Extraction and Separation of f- Block Elements

Autori: Petr Distler, Miriam Mindová, Jan John, Vasilij A. Babain, Mikhail Yu. Alyapyshev, Lyudmila I. Tkachenko, Ekaterina V. Kenf, Laurence M. Harwood, Ashfaq Afsar
Pubblicato in: Solvent Extraction and Ion Exchange, Numero 38/2, 2020, Pagina/e 180-193, ISSN 0736-6299
Editore: Marcel Dekker Inc.
DOI: 10.1080/07366299.2019.1708004

Stability of Different BTBP and BTPhen Extracting or Masking Compounds Against Gamma Radiation

Autori: Distler P., Mindova M., Šebesta J., Grűner B., Bavol D., Egberink R. J. M., Verboom W., Babain V. A., John J.,
Pubblicato in: Chemistry Research, Numero 24 issues/ year, 2021, Pagina/e 19 MS pages, ISSN 1520-5045
Editore: American Chemical Society

The conversion of ammonium uranate prepared via sol-gel synthesis into uranium oxides

Autori: Christian Schreinemachers, Gregory Leinders, Giuseppe Modolo, Marc Verwerft, Koen Binnemans, Thomas Cardinaels
Pubblicato in: Nuclear Engineering and Technology, Numero 52/5, 2020, Pagina/e 1013-1021, ISSN 1738-5733
Editore: Korean Nuclear Society
DOI: 10.1016/j.net.2019.11.004

Separation of Minor Actinides from Lanthanides Using Immobilized Ligand Systems: The Role of the Counterion

Autori: Laurence M. Harwood, Ashfaq Afsar, Petr Distler, Jan John, Jasraj S. Babra, Zoe Y. Selfe, Joeseph Cowell, James Westwood
Pubblicato in: HETEROCYCLES, Numero 99/2, 2019, Pagina/e 825, ISSN 0385-5414
Editore: Elsevier BV
DOI: 10.3987/com-18-s(f)71

Structural changes of Nd- and Ce-doped ammonium diuranate microspheres during the conversion to U1−LnO2±

Autori: Christian Schreinemachers, Gregory Leinders, Renaud Podor, Joseph Lautru, Nicolas Clavier, Giuseppe Modolo, Marc Verwerft, Koen Binnemans, Thomas Cardinaels
Pubblicato in: Journal of Nuclear Materials, Numero 542, 2020, Pagina/e 152454, ISSN 0022-3115
Editore: Elsevier BV
DOI: 10.1016/j.jnucmat.2020.152454

Solvent Extraction Investigations on Pu(IV) and Th(IV) Complexes with Hydrophilic SO 3 -Ph-BTP and SO 3 -Ph-BTBP Ligands

Autori: Łukasz Steczek, Jerzy Narbutt, Marie-Christine Charbonnel, Philippe Moisy
Pubblicato in: Solvent Extraction and Ion Exchange, Numero 37/3-4, 2019, Pagina/e 259-268, ISSN 0736-6299
Editore: Marcel Dekker Inc.
DOI: 10.1080/07366299.2019.1639366

A Study of Cerium Extraction Kinetics by TODGA in Acidified and Non-Acidified Organic Solvent Phases in the Context of Fission Product Management

Autori: Michael Anthony Bromley Colin Boxall
Pubblicato in: Progress in Nuclear Science and Technology, 2018, Pagina/e 70-73, ISSN 2185-4823
Editore: Atomic Energy Society of Japan
DOI: 10.15669/pnst.5.70

On the Basic Extraction Properties of a Phenyl Trifluoromethyl Sulfone-Based GANEX System Containing CyMe 4 -BTBP and TBP

Autori: Jenny Halleröd, Christian Ekberg, Thea Authen, Laura Bertolo, Mu Lin, Bohumír Grüner, Jaroslav Švehla, Christoph Wagner, Andreas Geist, Petra Panak, Emma Aneheim
Pubblicato in: Solvent Extraction and Ion Exchange, Numero 36/4, 2018, Pagina/e 360-372, ISSN 0736-6299
Editore: Marcel Dekker Inc.
DOI: 10.1080/07366299.2018.1497043

Radiolytic and hydrolytic degradation of the hydrophilic diglycolamides

Autori: Andreas Wilden, Bruce J. Mincher, Stephen P. Mezyk, Liam Twight, Kristyn M. Rosciolo-Johnson, Christopher A. Zarzana, Mary E. Case, Michelle Hupert, Andrea Stärk, Giuseppe Modolo
Pubblicato in: Solvent Extraction and Ion Exchange, Numero 36/4, 2018, Pagina/e 347-359, ISSN 0736-6299
Editore: Marcel Dekker Inc.
DOI: 10.1080/07366299.2018.1495384

Stoichiometry of An( iii )–DMDOHEMA complexes formed during solvent extraction

Autori: Patrik Weßling, Michael Trumm, Andreas Geist, Petra J. Panak
Pubblicato in: Dalton Transactions, Numero 47/32, 2018, Pagina/e 10906-10914, ISSN 1477-9226
Editore: Royal Society of Chemistry
DOI: 10.1039/c8dt02504e

Modified diglycolamides for grouped actinide separation

Autori: Rikard Malmbeck, Daniel Magnusson, Andreas Geist
Pubblicato in: Journal of Radioanalytical and Nuclear Chemistry, Numero 314/3, 2017, Pagina/e 2531-2538, ISSN 0236-5731
Editore: Akademiai Kiado
DOI: 10.1007/s10967-017-5614-2

Optimization and Single-Stage Centrifugal Contactor Experiments with the Novel Hydrophilic Complexant PyTri-Diol for the i -SANEX Process

Autori: Eros Mossini, Elena Macerata, Andreas Wilden, Peter Kaufholz, Giuseppe Modolo, Nicolò Iotti, Alessandro Casnati, Andreas Geist, Mario Mariani
Pubblicato in: Solvent Extraction and Ion Exchange, Numero 36/4, 2018, Pagina/e 373-386, ISSN 0736-6299
Editore: Marcel Dekker Inc.
DOI: 10.1080/07366299.2018.1507134

Behaviour of the extractant Me-TODGA upon gamma irradiation: quantification of degradation compounds and individual influences on complexation and extraction

Autori: V. Hubscher-Bruder, V. Mogilireddy, S. Michel, A. Leoncini, J. Huskens, W. Verboom, H. Galán, A. Núñez, J. Cobos, G. Modolo, A. Wilden, H. Schmidt, M.-C. Charbonnel, P. Guilbaud, N. Boubals
Pubblicato in: New Journal of Chemistry, Numero 41/22, 2017, Pagina/e 13700-13711, ISSN 1144-0546
Editore: Royal Society of Chemistry
DOI: 10.1039/c7nj02136d

Synthesis of size-controlled UO 2 microspheres from the hydrothermal conversion of U( iv ) aspartate

Autori: V. Trillaud, J. Maynadié, J. Manaud, J. Hidalgo, D. Meyer, R. Podor, N. Dacheux, N. Clavier
Pubblicato in: CrystEngComm, Numero 20/48, 2018, Pagina/e 7749-7760, ISSN 1466-8033
Editore: Royal Society of Chemistry
DOI: 10.1039/c8ce01352g

2,6-Bis(1-alkyl-1H-1,2,3-triazol-4-yl)-pyridines: selective lipophilic chelating ligands for minor actinides

Autori: Annalisa Ossola, Elena Macerata, Eros Mossini, Marco Giola, Maria Chiara Gullo, Arturo Arduini, Alessandro Casnati, Mario Mariani
Pubblicato in: Journal of Radioanalytical and Nuclear Chemistry, Numero 318/3, 2018, Pagina/e 2013-2022, ISSN 0236-5731
Editore: Akademiai Kiado
DOI: 10.1007/s10967-018-6253-y

Application of quantum mechanical simulations for studying the radiolytic stability of prospective extractants in the nuclear fuel cycle

Autori: Tomáš Koubský, Jakub Luštinec
Pubblicato in: Journal of Radioanalytical and Nuclear Chemistry, Numero 318/3, 2018, Pagina/e 2407-2413, ISSN 0236-5731
Editore: Akademiai Kiado
DOI: 10.1007/s10967-018-6225-2

Extraction Properties of 4-Tetra(hydroxyphenyl)BTPhen in Liquid-Liquid Extraction Systems with Cyclohexanone/Octanol or in a Solid-Phase Extraction System

Autori: Laurence M. Harwood, Jan John, Ashfaq Afsar, Jasraj S. Babra, Petr Distler, Iain Hopkins, James Westwood, Zoe Y. Selfe
Pubblicato in: HETEROCYCLES, Numero 101/1, 2020, Pagina/e 209, ISSN 0385-5414
Editore: Elsevier BV
DOI: 10.3987/com-19-s(f)14

Thermodynamic parameters of Am(III), Cm(III) and Eu(III) extraction by CyMe4-BTPhen in cyclohexanone from HNO3 solutions

Autori: Petr Distler, Karel Stamberg, Jan John, Laurence M. Harwood, Frank W. Lewis
Pubblicato in: The Journal of Chemical Thermodynamics, Numero 141, 2020, Pagina/e 105955, ISSN 0021-9614
Editore: Academic Press
DOI: 10.1016/j.jct.2019.105955

Activation of the Aromatic Core of 3,3′-(Pyridine-2,6-diylbis(1 H -1,2,3-triazole-4,1-diyl))bis(propan-1-ol)—Effects on Extraction Performance, Stability Constants, and Basicity

Autori: Patrik Weßling, Michael Trumm, Elena Macerata, Annalisa Ossola, Eros Mossini, Maria Chiara Gullo, Arturo Arduini, Alessandro Casnati, Mario Mariani, Christian Adam, Andreas Geist, Petra J. Panak
Pubblicato in: Inorganic Chemistry, Numero 58/21, 2019, Pagina/e 14642-14651, ISSN 0020-1669
Editore: American Chemical Society
DOI: 10.1021/acs.inorgchem.9b02325

On the basic extraction properties of a phenyl trifuoromethyl sulfone based GANEX system containing CyMe4-BTBP and TBP.

Autori: J. Halleröd, Ch. Ekberg, T. Authen, L. Bertolo, Mu Lin, B. Grüner, J. Švehla, Ch. Wagner, A. Geist, P. Panak, E. Aneheim.
Pubblicato in: Solvent Extraction and Ion Exchange, Numero Vol. 36, Numero 4, 2018, Pagina/e 360-372, ISSN 0736-6299
Editore: Marcel Dekker Inc.
DOI: 10.1080/07366299.2018.1497043

Stability studies of GANEX system under different irradiation conditions

Autori: Iván Sánchez-García, Hitos Galán, Jose Manuel Perlado, Joaquín Cobos
Pubblicato in: EPJ Nuclear Sciences & Technologies, Numero 5, 2019, Pagina/e 19, ISSN 2491-9292
Editore: EDP Sciences
DOI: 10.1051/epjn/2019049

Do An( iii ) and Ln( iii ) ions form heteroleptic complexes with diglycolamide and hydrophilic BT(B)P ligands in solvent extraction systems? A spectroscopic and DFT study

Autori: Irena Herdzik-Koniecko, Christoph Wagner, Michael Trumm, Udo Müllich, Bernd Schimmelpfennig, Jerzy Narbutt, Andreas Geist, Petra J. Panak
Pubblicato in: New Journal of Chemistry, Numero 43/16, 2019, Pagina/e 6314-6322, ISSN 1144-0546
Editore: Royal Society of Chemistry
DOI: 10.1039/c9nj00651f

Gamma and pulsed electron radiolysis studies of CyMe4BTBP and CyMe4BTPhen: identification of radiolysis products and effects on the hydrometallurgical separation of trivalent actinides and lanthanides

Autori: Schmidt H., Wilden* A., Modolo G., Bosbach D., Santiago-Schübel B., HupertM., Mincher B. J., Mezyk S. P., Švehla J., Grüner B., Ekberg Ch.,
Pubblicato in: Radiation Phys. Chem., Numero 12 issues/ year, 2021, Pagina/e 31 pp., ISSN 0969-806X
Editore: Pergamon Press Ltd.

Evaluation of the Hydrophilic Complexant N,N,N’,N’ -tetraethyldiglycolamide (TEDGA) and its Methyl-substituted Analogues in the Selective Am(III) Separation

Autori: Larissa Klaß, Andreas Wilden, Fabian Kreft, Christoph Wagner, Andreas Geist, Petra J. Panak, Irena Herdzik-Koniecko, Jerzy Narbutt, Giuseppe Modolo
Pubblicato in: Solvent Extraction and Ion Exchange, Numero 37/5, 2019, Pagina/e 297-312, ISSN 0736-6299
Editore: Marcel Dekker Inc.
DOI: 10.1080/07366299.2019.1651039

Fabrication of Nd- and Ce-doped uranium dioxide microspheres via internal gelation

Autori: Christian Schreinemachers; Gregory Leinders; Giuseppe Modolo; Marc Verwerft; Koen Binnemans; Thomas Cardinaels
Pubblicato in: Journal of Nuclear Materials, Numero 21, 2020, ISSN 0022-3115
Editore: Elsevier BV

Solvent Extraction for Nuclear Power

Autori: Jerzy Narbutt
Pubblicato in: Liquid-Phase Extraction, Numero Handbooks in Separation Science, Colin F. Poole, Editor, 2020, Pagina/e 725-744, ISBN 9780128169117
Editore: Elsevier
DOI: 10.1016/b978-0-12-816911-7.00024-4

The use of synergistic effects of lipophilic modifiers of TODGA-containing organic phase for improving separation of Am(III) from the early lanthanides in the process of stripping the metals with hydrophilic ligands. A novel concept for solving the problem

Autori: Jerzy Narbutt, Irena Herdzik-Koniecko, Magdalena Rejnis-Strzelak
Pubblicato in: RAPORTY IChTJ, SERIA B, Numero Nr 2/2017, 2017, Pagina/e 1 - 14, ISSN 1425-7351
Editore: ICHTJ

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