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MultiphasIc NanoreaCtors for HEterogeneous CataLysis via SmArt ENGinEering of TaiLored DispersiOns

Ziel

Gas-liquid-solid (G/L/S) multiphasic reactors are extensively used in the chemical industry for catalytic processes. However, conventional reactors, such as packed beds and slurry reactors, typically suffer from resilient mass/heat transfer limitations due to their low specific interface areas, long mixing times, and a reduced accessibility of the gas reactants to the catalyst surface. To overcome these limitations, continuous flow microreactors and catalytic membrane reactors have been considered for increasing the G/L interface area, but these systems require complex equipment and still do not guarantee an efficient L/S contact at the catalyst surface. For a major improvement on current systems in terms of cost efficiency and energy savings, G/L/S reactors operating at the nanoscale are required.
The aim of this ERC project is to design robust particle-stabilized G/L dispersions (i.e. micro/nano-bubbles and liquid marbles) as highly efficient G/L/S nanoreactors for conducting catalytic reactions at mild conditions.

We will (i) prepare NPs with defined sizes, shapes, hydrophilic-lipophilic balance (HLB), including catalytic functions; (ii) generate particle-stabilized bubbles and liquid marbles affording highly active and selective reactions at the G/L/S interface with NP recycling after each catalytic cycle using external stimuli; examine the interplay between the NP assembly at the G/L interface and the catalytic properties along the reaction by combining well-designed experiments with simulations; and (iv) reengineer G/L/S multiphasic reactors using our particle-stabilized nanoreactors to achieve a high catalytic performance at milder operation conditions compared to conventional reactors while keeping a high degree of stability and flexibility at reduced layouts.

Through innovation on both amphiphilic catalysts and process intensification, MICHELANGELO will deliver a radical step change towards a higher efficiency and competitiveness in the process industry.

Gastgebende Einrichtung

CARDIFF UNIVERSITY
Netto-EU-Beitrag
€ 1 309 330,91
Adresse
NEWPORT ROAD 30 36
CF24 0DE Cardiff
Vereinigtes Königreich

Auf der Karte ansehen

Region
Wales East Wales Cardiff and Vale of Glamorgan
Aktivitätstyp
Higher or Secondary Education Establishments
Links
Gesamtkosten
€ 1 309 330,91

Begünstigte (2)