Catalytic cascade reactions. From fundamentals of nanozymes to applications based on gas-diffusion electrodes

Pubblicazioni

Calibrating SECCM measurements by means of a nanoelectrode ruler. The intrinsic oxygen reduction activity of PtNi catalyst nanoparticles

Autori: Emmanuel Batsa Tetteh, Tobias Löffler, Tsvetan Tarnev, Thomas Quast, Patrick Wilde, Harshitha Barike Aiyappa, Simon Schumacher, Corina Andronescu, Richard D. Tilley, Xingxing Chen, Wolfgang Schuhmann,
Pubblicato in: Nano Research, Numero 15, 2022, Pagina/e 1564-1569, ISSN 1998-0124
Editore: Tsinghua Univ Press
DOI: 10.1007/s12274-021-3702-7

Zooming-in – Visualization of active site heterogeneity in high entropy alloy electrocatalysts using scanning electrochemical cell microscopy

Autori: Emmanuel Batsa Tetteh; Lars Banko; Olga A. Krysiak; Tobias Löffler; Bin Xiao; Swapnil Varhade; Simon Schumacher; Alan Savan; Corina Andronescu; Alfred Ludwig; Wolfgang Schuhmann
Pubblicato in: Electrochemical Science Advances, Numero 2, 2021, Pagina/e e2100105, ISSN 2698-5977
Editore: Wiley-VCH GmbH
DOI: 10.1002/elsa.202100105

A Flexible Theory for Catalysis: Learning Alkaline Oxygen Reduction on Complex Solid Solutions within the Ag−Pd−Pt−Ru Composition Space

Autori: Christian M. Clausen, Olga A. Krysiak, Lars Banko, Jack K. Pedersen, Wolfgang Schuhmann, Alfred Ludwig, Jan Rossmeisl
Pubblicato in: Angewandte Chemie International Edition, Numero 62, 2023, Pagina/e e202307187, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202307187

Simultaneous Anodic and Cathodic Formate Production in a Paired Electrolyzer by CO2 Reduction and Glycerol Oxidation

Autori: João R. C. Junqueira, Debanjan Das, Ann Cathrin Brix, Stefan Dieckhöfer, Jonas Weidner, Xin Wang, Jialin Shi, Wolfgang Schuhmann
Pubblicato in: ChemSusChem, Numero 16, 2024, Pagina/e e202202349, ISSN 1864-5631
Editore: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1002/cssc.202202349

Hollow CeO 2 @Co 2 N Nanosheets Derived from Co‐ZIF‐L for Boosting the Oxygen Evolution Reaction

Autori: Jian Zhang, Wenhui He, Harshitha Barike Aiyappa, Thomas Quast, Stefan Dieckhöfer, Denis Öhl, João R. C. Junqueira, Yen‐Ting Chen, Justus Masa, Wolfgang Schuhmann
Pubblicato in: Advanced Materials Interfaces, Numero 8/9, 2021, Pagina/e 2100041, ISSN 2196-7350
Editore: Wiley-VCH
DOI: 10.1002/admi.202100041

Bayesian Optimization of High-Entropy Alloy Compositions for Electrocatalytic Oxygen Reduction

Autori: Jack K. Pedersen, Christian M. Clausen, Olga A. Krysiak, Bin Xiao, Thomas A. A. Batchelor, Tobias Löffler, Vladislav A. Mints, Lars Banko, Matthias Arenz, Alan Savan, Wolfgang Schuhmann, Alfred Ludwig, Jan Rossmeisl
Pubblicato in: Angewandte Chemie International Edition, Numero 60, 2021, Pagina/e 24144-24152, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202108116

Discovery of High-Entropy Oxide Electrocatalysts: From Thin-Film Material Libraries to Particles

Autori: Strotkötter, Valerie; Krysiak, Olga A.; Zhang, Jian; Wang, Xiao; Suhr, Ellen; Schuhmann, Wolfgang; Ludwig, Alfred
Pubblicato in: Chemistry of Materials, Numero 34, 2022, Pagina/e 10291−10303, ISSN 0897-4756
Editore: American Chemical Society
DOI: 10.1021/acs.chemmater.2c01455

Differentiation between Carbon Corrosion and Oxygen Evolution Catalyzed by Ni x B/C Hybrid Electrocatalysts in Alkaline Solution using Differential Electrochemical Mass Spectrometry

Autori: Sandra Möller, Stefan Barwe, Stefan Dieckhöfer, Justus Masa, Corina Andronescu, Wolfgang Schuhmann
Pubblicato in: ChemElectroChem, Numero 7/12, 2020, Pagina/e 2680-2686, ISSN 2196-0216
Editore: Wiley-VCH Verlag GmbH &Co. KGaA
DOI: 10.1002/celc.202000697

Single Particle Nanoelectrochemistry Reveals the Catalytic Oxygen Evolution Reaction Activity of Co 3 O 4 Nanocubes

Autori: Thomas Quast, Swapnil Varhade, Sascha Saddeler, Yen‐Ting Chen, Corina Andronescu, Stephan Schulz, Wolfgang Schuhmann
Pubblicato in: Angewandte Chemie International Edition, Numero 60/43, 2021, Pagina/e 23444-23450, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202109201

Cascade Reactions in Nanozymes: Spatially Separated Active Sites inside Ag-Core–Porous-Cu-Shell Nanoparticles for Multistep Carbon Dioxide Reduction to Higher Organic Molecules

Autori: Peter B. O’Mara, Patrick Wilde, Tania M. Benedetti, Corina Andronescu, Soshan Cheong, J. Justin Gooding, Richard D. Tilley, Wolfgang Schuhmann
Pubblicato in: Journal of the American Chemical Society, Numero 141/36, 2019, Pagina/e 14093-14097, ISSN 0002-7863
Editore: American Chemical Society
DOI: 10.1021/jacs.9b07310

Ag-induced Phase Transition of Bi2O3 Nanofibers for Enhanced Energy Conversion Efficiency towards Formate in CO2 Electroreduction

Autori: Wang, Xin; He, Wenhui; Shi, Jialin; Junqueira, João R. C.; Zhang, Jian; Dieckhöfer, Stefan; Seisel, Sabine; Das, Debanjan; Schuhmann, Wolfgang
Pubblicato in: Chemistry - an Asian Journal, Numero 18, 2023, Pagina/e e202201165, ISSN 1861-4728
Editore: Wiley - V C H Verlag GmbbH & Co.
DOI: 10.1002/asia.202201165

A Universal Nano‐capillary Based Method of Catalyst Immobilization for Liquid‐Cell Transmission Electron Microscopy

Autori: Tsvetan Tarnev, Steffen Cychy, Corina Andronescu, Martin Muhler, Wolfgang Schuhmann, Yen‐Ting Chen
Pubblicato in: Angewandte Chemie International Edition, Numero 59/14, 2020, Pagina/e 5586-5590, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.201916419

Single-entity Electrochemistry Unveils Dynamic Transformation during Tandem Catalysis of Cu2O and Co3O4 for Converting NO3- to NH3

Autori: Zhang, Jian; He, Wenhui; Quast, Thomas; Junqueira, João R. C.; Saddeler, Sascha; Schulz, Stephan; Schuhmann, Wolfgang
Pubblicato in: Angewandte Chemie - International Edition, Numero 62, 2022, Pagina/e e202214830, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202214830

Nanoconfinement Allows a Less Active Cascade Catalyst to ProduceMore C2+ Products in Electrochemical CO2 Reductio

Autori: Samuel V. Somerville, Peter B. O’Mara, Tania M. Benedetti, Soshan Cheong, Wolfgang Schuhmann, Richard D. Tilley, J. Justin Gooding
Pubblicato in: Journal of Physical Chemistry C, Numero 127, 2023, Pagina/e 289-299, ISSN 1932-7447
Editore: American Chemical Society
DOI: 10.1021/acs.jpcc.2c07518

Probing the Local Reaction Environment During High Turnover Carbon Dioxide Reduction with Ag‐Based Gas Diffusion Electrodes

Autori: Stefan Dieckhöfer, Denis Öhl, João R. C. Junqueira, Thomas Quast, Thomas Turek, Wolfgang Schuhmann
Pubblicato in: Chemistry – A European Journal, Numero 27/19, 2021, Pagina/e 5906-5912, ISSN 0947-6539
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/chem.202100387

A Metal–Organic Framework derived Cu x O y C z Catalyst for Electrochemical CO 2 Reduction and Impact of Local pH Change

Autori: Nivedita Sikdar, João R. C. Junqueira, Stefan Dieckhöfer, Thomas Quast, Michael Braun, Yanfang Song, Harshitha B. Aiyappa, Sabine Seisel, Jonas Weidner, Denis Öhl, Corina Andronescu, Wolfgang Schuhmann
Pubblicato in: Angewandte Chemie International Edition, Numero 60/43, 2021, Pagina/e 23427-23434, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202108313

Electroenzymatic Nitrogen Fixation Using a MoFe Protein System Immobilized in an Organic Redox Polymer

Autori: Yoo Seok Lee, Adrian Ruff, Rong Cai, Koun Lim, Wolfgang Schuhmann, Shelley D. Minteer
Pubblicato in: Angewandte Chemie International Edition, Numero 59/38, 2020, Pagina/e 16511-16516, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202007198

Splicing the active phases of copper/cobalt-based catalysts achieves high-rate tandem electroreduction of nitrate to ammonia

Autori: Wenhui He, Jian Zhang, Stefan Dieckhöfer, Swapnil Varhade, Ann Cathrin Brix, Anna Lielpetere, Sabine Seisel , João R. C. Junqueira, Wolfgang Schuhmann
Pubblicato in: Nature Communications, Numero 13, 2022, Pagina/e 1129, ISSN 2041-1723
Editore: Nature Publishing Group
DOI: 10.1038/s41467-022-28728-4

Electrocatalysis as the Nexus for Sustainable Renewable Energy: The Gordian Knot of Activity, Stability, and Selectivity

Autori: Justus Masa, Corina Andronescu, Wolfgang Schuhmann
Pubblicato in: Angewandte Chemie International Edition, Numero 59/36, 2020, Pagina/e 15298-15312, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202007672

High-Throughput Exploration of Structural and Electrochemical Properties of the High-Entropy Nitride System (Ti–Co–Mo–Ta–W)N

Autori: Ellen Suhr, Olga A. Krysiak, Valerie Strotkötter, Felix Thelen, Wolfgang Schuhmann, Alfred Ludwig
Pubblicato in: Advanced Engineering Materials, Numero 25, 2023, Pagina/e 2300550, ISSN 1438-1656
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/adem.202300550

Revealing the Heterogeneity of Large-Area MoS2 Layers in the Electrocatalytic Hydrogen Evolution Reaction

Autori: Schumacher, Simon; Madauß, Lukas; Liebsch, Yossarian; Batsa Tetteh, Emmanuel; Varhade, Swapnil; Schuhmann, Wolfgang; Schleberger, Marika; Andronescu, Corina
Pubblicato in: ChemElectroChem, Numero 21960216, 2022, Pagina/e e202200586, ISSN 2196-0216
Editore: Wiley-VCH
DOI: 10.1002/celc.202200586

Complex‐Solid‐Solution Electrocatalyst Discovery by Computational Prediction and High‐Throughput Experimentation**

Autori: Thomas A. A. Batchelor, Tobias Löffler, Bin Xiao, Olga A. Krysiak, Valerie Strotkötter, Jack K. Pedersen, Christian M. Clausen, Alan Savan, Yujiao Li, Wolfgang Schuhmann, Jan Rossmeisl, Alfred Ludwig
Pubblicato in: Angewandte Chemie International Edition, Numero 60/13, 2021, Pagina/e 6932-6937, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202014374

Influence of the PTFE Membrane Thickness on the CO2 Electroreduction Performance of Sputtered Cu-PTFE Gas Diffusion Electrodes

Autori: Huq, Faria; Sanjuán, Ignacio; Baha, Sabrina; Braun, Michael; Kostka, Aleksander; Chanda, Vimanshu; Junqueira, João R. C.; Sikdar, Nivedita; Ludwig, Alfred; Andronescu, Corina
Pubblicato in: ChemElectroChem, Numero 21960216, 2022, Pagina/e e202101279, ISSN 2196-0216
Editore: Wiley-VCH
DOI: 10.1002/celc.202101279

Operando Scanning Electrochemical Probe Microscopy during Electrocatalysis

Autori: Santana Santos, Carla; Jaato, Bright Nsolebna; Sanjuán, Ignacio; Schuhmann, Wolfgang; Andronescu, Corina
Pubblicato in: ACS - Chemical Reviews, Numero 123, 2023, Pagina/e 4972–5019, ISSN 0009-2665
Editore: American Chemical Society
DOI: 10.1021/acs.chemrev.2c00766

Sprayed Ag oxygen reduction reaction gas-diffusion electrodes for the electrocatalytic reduction of CO2 to CO

Autori: Wilde, Patrick; Özden, Anil; Winter, Henrik; Quast, Thomas; Weidner, Jonas; Dieckhöfer, Stefan; Junqueira, João R. C.; Metzner, Matthias; Peter, Willi; Leske, Werner; Öhl, Denis; Bobrowski, Tim; Turek, Thomas; Schuhmann, Wolfgang
Pubblicato in: Applied Research, Numero 2, 2022, Pagina/e e202200081, ISSN 2702-4288
Editore: Wiley-VCH GmbH
DOI: 10.1002/appl.202200081

Acidic Hydrogen Evolution Electrocatalysis at High-Entropy Alloys Correlates with its Composition-Dependent Potential of Zero Charge

Autori: Moonjoo Kim, Emmanuel Batsa Tetteh, Olga A. Krysiak, Alan Savan, Dr. Bin Xiao, Tobias Horst Piotrowiak, Corina Andronescu, Alfred Ludwig, Taek Dong Chung, Wolfgang Schuhmann
Pubblicato in: Angewandte Chemie International Edition, Numero 62, 2023, Pagina/e e202310069, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202310069

Is Cu instability during the CO 2 reduction reaction governed by the applied potential or the local CO concentration?

Autori: Patrick Wilde, Peter B. O'Mara, João R. C. Junqueira, Tsvetan Tarnev, Tania M. Benedetti, Corina Andronescu, Yen-Ting Chen, Richard D. Tilley, Wolfgang Schuhmann, J. Justin Gooding
Pubblicato in: Chemical Science, Numero 12/11, 2021, Pagina/e 4028-4033, ISSN 2041-6520
Editore: Royal Society of Chemistry
DOI: 10.1039/d0sc05990k

Microscale Combinatorial Libraries for the Discovery of High-Entropy Materials

Autori: Banko, Lars; Batsa Tetteh, Emmanuel; Kostka, Aleksander; Piotrowiak, Tobias Horst; Krysiak, Olga Anna; Hagemann, Ulrich; Andronescu, Corina; Schuhmann, Wolfgang; Ludwig, Alfred
Pubblicato in: Advanced Materials, 2023, ISSN 1521-4095
Editore: Wiley-VCH GmbH
DOI: 10.1002/adma.202207635

In Situ Carbon Corrosion and Cu Leaching as a Strategy for Boosting Oxygen Evolution Reaction in Multimetal Electrocatalysts

Autori: Jian Zhang, Thomas Quast, Wenhui He, Stefan Dieckhöfer, João R. C. Junqueira, Denis Öhl, Patrick Wilde, Daliborka Jambrec, Yen-Ting Chen, Wolfgang Schuhmann
Pubblicato in: Advanced Materials, 2022, Pagina/e 2109108, ISSN 1521-4095
Editore: Wiley-VCH GmbH
DOI: 10.1002/adma.202109108

Searching novel complex solid solution electrocatalysts in unconventional element combinations

Autori: Olga A. Krysiak, Simon Schumacher, Alan Savan, Wolfgang Schuhmann, Alfred Ludwig, Corina Andronescu
Pubblicato in: Nano Research volume, Numero 15, 2022, Pagina/e 4780–4784, ISSN 1998-0124
Editore: Tsinghua Univ Press
DOI: 10.1007/s12274-021-3637-z

Dynamic Transformation of Functionalized Bismuth to Catalytically Active Surfaces for CO2 Reduction to Formate at High Current Densities

Autori: Muhammad Adib Abdillah Mahbub, João R. C. Junqueira, Xin Wang, Jian Zhang, Stefan Dieckhöfer, Sabine Seisel, Debanjan Das, Wolfgang Schuhmann
Pubblicato in: Advanced Functional Materials, Numero 34, 2024, Pagina/e 2307752, ISSN 1616-301X
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/adfm.202307752

B‐Cu‐Zn Gas Diffusion Electrodes for CO 2 Electroreduction to C 2+ Products at High Current Densities

Autori: Yanfang Song, João R. C. Junqueira, Nivedita Sikdar, Denis Öhl, Stefan Dieckhöfer, Thomas Quast, Sabine Seisel, Justus Masa, Corina Andronescu, Wolfgang Schuhmann
Pubblicato in: Angewandte Chemie International Edition, Numero 60/16, 2021, Pagina/e 9135-9141, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202016898

Enhanced Nitrate-to-Ammonia Efficiency over Linear Assemblies of Copper-Cobalt Nanophases Stabilized by Redox Polymers

Autori: Wenhui He, Shubhadeep Chandra, Thomas Quast, Swapnil Varhade, Stefan Dieckhöfer, João R. C. Junqueira, Huimin Gao, Sabine Seisel, and Wolfgang Schuhman
Pubblicato in: Advanced Materials, Numero 35, 2023, Pagina/e 2303050, ISSN 0935-9648
Editore: United Nations Industrial Developement Organization
DOI: 10.1002/adma.202303050

Probing the local activity of CO2 reduction on gold gas diffusion electrodes: effect of the catalyst loading and CO2 pressure

Autori: Mariana C. O. Monteiro, Stefan Dieckhöfer, Tim Bobrowski, Thomas Quast, Davide Pavesi, Marc T.M. Koper, Wolfgang Schuhmann
Pubblicato in: Chemical Science, Numero 12, 2021, Pagina/e 15682-15690, ISSN 2041-6539
Editore: Royal Society of Chemistry
DOI: 10.1039/d1sc05519d

Gaining the Freedom of Scalable Gas Diffusion Electrodes for the CO2 Reduction Reaction

Autori: Wang, Xin; Tomon, Chanikarn; Bobrowski, Tim; Wilde, Patrick; Junqueira, João R. C.; Quast, Thomas; He, Wenhui; Sikdar, Nivedita; Weidner, Jonas; Schuhmann, Wolfgang
Pubblicato in: ChemElectroChem, Numero 9, 2022, Pagina/e e202200675, ISSN 2196-0216
Editore: Wiley-VCH
DOI: 10.1002/celc.202200675

Single‐Entity Electrocatalysis of Individual “Picked‐and‐Dropped” Co 3 O 4 Nanoparticles on the Tip of a Carbon Nanoelectrode

Autori: Thomas Quast, Harshitha Barike Aiyappa, Sascha Saddeler, Patrick Wilde, Yen‐Ting Chen, Stephan Schulz, Wolfgang Schuhmann
Pubblicato in: Angewandte Chemie International Edition, Numero 60/7, 2021, Pagina/e 3576-3580, ISSN 1433-7851
Editore: John Wiley & Sons Ltd.
DOI: 10.1002/anie.202014384

Redox Replacement of Silver on MOF-Derived Cu/C Nanoparticles on Gas Diffusion Electrodes for Electrocatalytic CO2 Reduction

Autori: Nivedita Sikdar, João R. C. Junqueira, Denis Öhl, Stefan Dieckhöfer, Thomas Quast, Michael Braun, Harshitha B. Aiyappa, Sabine Seisel, Corina Andronescu, Wolfgang Schuhmann
Pubblicato in: Chemistry - A European Journal, Numero 28, 2022, Pagina/e e20210424, ISSN 1521-3765
Editore: Wiley-VCH GmbH
DOI: 10.1002/chem.202104249

Combining Nanoconfinement in Ag Core/Porous Cu Shell Nanoparticles with Gas Diffusion Electrodes for Improved Electrocatalytic Carbon Dioxide Reduction

Autori: João R. C. Junqueira, Peter B. O'Mara, Patrick Wilde, Stefan Dieckhöfer, Tania M. Benedetti, Corina Andronescu, Richard D. Tilley, J. Justin Gooding, Wolfgang Schuhmann
Pubblicato in: ChemElektroChem, Numero 8, 2021, Pagina/e 4848-4853, ISSN 2196-0216
Editore: Wiley-VCH GmbH
DOI: 10.1002/celc.202100906

È in corso la ricerca di dati su OpenAIRE...

Pubblicazioni

Condividi questa pagina

Scarica