Carbon Captured Fuel and Energy Carriers for an Intensified Steel Off-Gases based Electricity Generation in a Smarter Industrial Ecosystem

Livrables

Influence of pressure on the single cells performance and durability

Results of electrochemical and microstructural analysis of a single cell under different operating pressures. Results of a 500 hours durability test at high pressure (subtask 2.2.4).

Multiscale modelling results

Results of the 0D and 3D SOE stack models developed in task 2.4 under steady and dynamic states. Delivery of a SOE stack model to integrate to the demonstration pilot model.

Technical workshop summary

Presentation of project first results WP1 to WP4 to a wide international audience task 74

Goal and scope of the LCA

Definition of goal and scope of the LCA. Creation of data collection templates to manage collection process (task 6.3).

Steel-off gases pre-treatment unit design

Definition of the pretreatment section required before CO2 conditioning step Integration of the gas treatment unit within demonstrator pilot subtask 121

Report on 5000 hours durability test of SOEC under relevant operation conditions

Results of electrochemical and microstructural analysis of a single cell operating under the previously identified optimal operation conditions. Conclusion on SOEC reliability for hydrogen and syngas production (subtask 2.2.6).

Study of social acceptance of the C2FUEL project (1)

Intermediate results of social acceptance of C2FUEL project. Partial communication analysis and first interviews report (task 7.1).

Catalyst synthetized for FA production

Results of tested catalysts for formic acid production. Definition of selected catalyst and results of high pressure operation and long term stability tests (task 4.2).

Preliminary Environmental assessment through LCA

Report of preliminary LCA to identify most significant environmental impacts and sensitive parameters (task 6.3).

Specifications for the demonstrator

Portfolio of all data gathered in task 11 and task 12 to define precisely the KPI of the demonstrator systems to be built within C2FUEL project

Electricity production and consumption in Dunkirk area

Analysis of Dunkirk area electricity sourcing. Assessment of renewable electricity surplus potential. Levelized cost forecast of both grid and renewable electricity (task 1.4).

Influence of operation conditions on single cells performance and durability

Identification of safe operation conditions range based on single cell tests Delivery of a suitable operation strategy to increase lifespan of single cells and SOE stacks subtask 221 Results of dynamic operation tests subtask 225

Influence of sweeping gases on the single cells performance and durability

Results of electrochemical impedance spectroscopy and post-test microstructure analysis of a single cell operating under different sweeping gases. Impact of sweeping gas on the oxygen electrode degradation (subtask 2.2.3).

Newsletters 3

External communication and dissemination of C2FUEL project results task 73

Project website

A public project website will be set up by M6 by ENGIE in order to widely communicate and disseminate project results (task 7.3).

Newsletters 1

Communication through project documentation, media and local newspapers to measure social acceptance of the project. Organisation of an interview survey with local stakeholders (task 7.1).

Newsletters 2

Organized workshops to establish a first mapping of key stakeholders. Communication through providing and sharing of scientific information as well as action coordination (task 7.2).

Publications

Presentation of C2FUEL project

Auteurs: P. Olivier, C. Makhloufi
Publié dans: 2020
Éditeur: INEA

In2O3 nanoparticles Gas Diffusion Electrode (GDE) (oral)

Auteurs: Marta C. Figueiredo
Publié dans: Annual Meeting of the Danish Electrochemical society - 29/10/20, 2020
Éditeur: Danish Electrochemical societ

Presentation of C2FUEL project

Auteurs: P. Olivier, C. Makhloufi, M. Marrot
Publié dans: 4th INEA workshop on CCUS (sept 2019), 2019
Éditeur: INEA

Poster: Effect of doping In2O3 with transition metals on the electrocatalytic reduction of CO2 to formate

Auteurs: Tim Wissink, Marta Figueiredo, Emiel Hensen
Publié dans: EcoCat conference 23-25/11/2020, 2020
Éditeur: NanoGe

Solid Oxide Electrolyser Demonstrator Development at Elcogen

Auteurs: Lehtinen, Timo; Noponen, Matti
Publié dans: 2021 Meet. Abstr. MA2021-03 285, Numéro 2, 2021
Éditeur: IOP Publishing
DOI: 10.1149/ma2021-031285mtgabs

EFFECT OF BOEHMITE NANOPARTICLES ON ALUMINA SUPPORTED CARBON MOLECULAR SIEVE MEMBRANES FOR VAPOR/GAS PERMEATION

Auteurs: SERENA POTO,MARGOT A. LLOSA TANCO, D. ALFREDO PACHECO TANAKA,FAUSTO GALLUCCI, M. FERNANDA NEIRA D’ANGELO
Publié dans: World Online Conference on Sustainable Technologies (WOCST), 2021
Éditeur: WOCST

Effect of membrane properties on the direct conversion of CO2 to dimethyl ether in a fixed bed membrane reactor

Auteurs: Serena Poto, Fausto Gallucci, M. Fernanda Neira d’Angelo
Publié dans: 11th International Symposium on Catalysis in Multiphase Reactors (CAMURE-11), 2021
Éditeur: AIDIC

PERFORMANCE CHARACTERISTICS OF SOLID OXIDE ELECTROLYSIS TECHNOLOGY FROM ELCOGEN

Auteurs: Timo Lehtinen, Matti Noponen, Sergii Pylypko and Enn Õunpuu
Publié dans: 45th International Conference and Expo on Advanced Ceramics and Composites (IACC), 2021
Éditeur: ACerS Engineering Ceramics Division

EFFECT OF MEMBRANE PROPERTIES ON THE DIRECT CONVERSION OF CO2 TO DIMETHYL ETHER IN A FIXED BED MEMBRANE REACTOR (oral)

Auteurs: SERENA POTO, FAUSTO GALLUCCI, M. FERNANDA NEIRA D’ANGELO
Publié dans: International Conference on Catalysis in Membrane Reactors (ICCMR-15), 2022
Éditeur: The membrane society of Japan

Kinetic modelling of the methanol synthesis from CO2 and H2 over a CuO/CeO2/ZrO2 catalyst: the role of CO2 and CO hydrogenation

Auteurs: Serena Poto, Damian Vico van Berkel, Fausto Gallucci, M. Fernanda Neira d’Angelo
Publié dans: North American Catalysis Society Meeting (NAM 27), 2022
Éditeur: NAM

Catalytic performance study of supported Au catalysts for the direct hydrogenation of CO2 to formic acid

Auteurs: Anouk de Leeuw den Bouter, Pierre Oliver, Camel Makhloufi, John van der Schaaf
Publié dans: Netherlands’ Catalysis and Chemistry Conference (NCCC), 2022
Éditeur: NCCC

Design of membrane based gas-liquid absorption units: a fast, efficient, high throughput batch to continuous methodology (abstract)

Auteurs: E. Ferreri, C. Castel, E. Favre
Publié dans: Euromembrane 2021, 2021
Éditeur: The Meeting Planners

Design of membrane based gas-liquid absorption units: a fast, efficient, high throughput batch to continuous methodology (oral)

Auteurs: Eglé FERRERI, Christophe CASTEL, Eric Favre
Publié dans: SFGP 2022, 2022
Éditeur: Société Française de Génie des Procédés

High temperature electrolysis and co-electrolysis

Auteurs: M. Noponen, Timo Lehtinen and X. Sun
Publié dans: C2Fuel workshop: International Workshop on CO2 capture and utilization, 2021
Éditeur: C2Fuel - TU/e

C2FUEL Solid Oxide Electrolyser Demonstration System

Auteurs: Timo Lehtinen, Matti Noponen
Publié dans: 15th European SOFC & SOE Forum, 2022
Éditeur: EFCF

Kinetic modelling of the methanol synthesis from CO2 and H2 over a CuO/CeO2/ZrO2 catalyst: the role of CO2 and CO hydrogenation

Auteurs: S. Poto, M.F. Neira d’Angelo, F. Gallucci
Publié dans: Netherlands’ Catalysis and Chemistry Conference (NCCC), 2022
Éditeur: NCCC

An industrially-relevant demonstration of a CCU-based circular economy (poster)

Auteurs: B. Wegman, F. Gallucci, P. Olivier, C. Makhloufi
Publié dans: C2Fuel workshop: International Workshop on CO2 capture and utilization, 2021
Éditeur: C2Fuel - TU/e

Morphology study of bismuth nanoparticles as catalyst for electrochemical CO2 reduction to formate (poster)

Auteurs: Alex J.W. Mana, Tim Wissinka, Marta C. Figueiredoa, Emiel J.M. Hensena
Publié dans: Netherlands’ Catalysis and Chemistry Conference (NCCC), 2022
Éditeur: NCCC

Degradation of solid oxide electrolysis cells under different operation conditions

Auteurs: Xiufu Sun, Peter Vang Hendriksen, Anne Hauch1, Anders Kring Clausen, Timo Lehtinen, Matti Noponen (abstract)
Publié dans: 17th International Symposium on Solid Oxide Fuel Cells (SOFC), 2021
Éditeur: The Electrochemical Society

Stability of In2O3 Nanoparticles in Gas Diffusion Electrodes for CO2 Reduction to Formate

Auteurs: Tim Wissink
Publié dans: Netherlands’ Catalysis and Chemistry Conference (NCCC), 2022
Éditeur: NCCC

Effect of doping In2O3 with transition metals on the electrocatalytic reduction of CO2 to formate (poster)

Auteurs: Tim Wissink, Marta C. Figueiredo, Emiel J.M. Hensen
Publié dans: C2Fuel workshop: International Workshop on CO2 capture and utilization, 2021
Éditeur: C2Fuel - TU/e

Stability of In2O3 Nanoparticles in PTFE-containing Gas Diffusion Electrodes for CO2 Electroreduction to formate

Auteurs: Tim Wissink, Rim C.J. Van de Poll, Dr. Marta C.C. Figueiredo,Prof. Emiel J.M. Hensen
Publié dans: MAT-SUS conference -Materials for Sustainable Development, 2022
Éditeur: nanoGe

Effect of the membrane properties on the direct conversion of CO2 to dimethyl ether in a fixed bed membrane reactor (oral)

Auteurs: S. Poto, M.F. Neira d’Angelo, F. Gallucci
Publié dans: North American Catalysis Society Meeting (NAM 27), 2022
Éditeur: NAM

EFFECT OF BOEHMITE NANOSHEETS ON ALUMINA SUPPORTED CARBON MOLECULAR SIEVE MEMBRANES FOR VAPOR/GAS PERMEATION: EXPERIMENTAL AND THEORETICAL INVESTIGATION (oral)

Auteurs: SERENA POTO, MARGOT A. LLOSA TANCO, D. ALFREDO PACHECO TANAK*, FAUSTO GALLUCCI, M. FERNANDA NEIRA D’ANGELO
Publié dans: International Conference on Catalysis in Membrane Reactors (ICCMR-15), 2022
Éditeur: The membrane society of Japan

PERFORMANCE CHARACTERISTICS OF SOLID OXIDE ELECTROLYSIS TECHNOLOGY FROM ELCOGEN (bstract + presentation video)

Transition metal doped In2O3 for CO2 reduction to formate: How to retain the oxide phase for improved stability

Auteurs: T. Wissink, M.C.C. Figuereido, E.J.M. Hensen
Publié dans: Netherlands’ Catalysis and Chemistry Conference (NCCC, 2022
Éditeur: NCCC

Effect of inlet gas composition on the durability of solid oxide electrolysis cells

Auteurs: Xiufu Sun, Anders Kring Clausen, Peter Vang Hendriksen, Anne Hauch, Timo Lehtinen, Matti Noponen
Publié dans: 2022
Éditeur: EFCF
DOI: 10.5281/zenodo.7846265

Presentation of C2FUEL project

Auteurs: Adeline Miquelot
Publié dans: COZMOS workshop on Conversion of CO2 to Fuels, 2023
Éditeur: COZMOS european project

Presentation of C2FUEL project

Auteurs: Bérenger WEGMAN
Publié dans: ENGIE AMEA, 2023
Éditeur: ENGIE

On-Site Demonstration of Pre-Combustion CO2 Capture from Industrial Blast-Furnace Gas with Heterogeneous Hollow-Fiber Contactor Membrane Absorption Modules

Auteurs: Bérenger WEGMAN, Eglé Ferreri
Publié dans: The 23rd IERE General Meeting and Singapore Forum, 2023
Éditeur: IERE

On the influence of trialkylamine reduction strategies in the direct hydrogenation of CO2 to formic acid (oral)

Auteurs: Anouk de Leeuw den Bouter, Lars Vogels, Esther Vogels, Pierre Olivier, Adeline Miquelot, Camel Makhloufi, John van der Schaaf
Publié dans: 2022 AIChE Annual Meeting, 2022
Éditeur: American Institute of Chemical Engineers.

Membrane contactors for CO2 capture and purification unit at demonstrator scale on industrial operating conditions (oral)

Auteurs: E. Ferreri
Publié dans: International Conference of Membrane 2023 (ICOM 2023), 2023
Éditeur: Membrane Society of Australasia

EFFECT OF CARBONIZATION TEMPERATURE ON THE gas PERMEATION OF ALUMINA-CARBON MOLECULAR SIEVE MEMBRANES (Al-CMSM)

Auteurs: MARGOT A. LLOSA TANCO, SERENA POTO, FAUSTO GALLUCCI,D. ALFREDO PACHECO TANAKA,
Publié dans: International Conference on Catalysis in Membrane Reactors (ICCMR-15), 2022
Éditeur: The membrane society of Japan

Effect of membrane properties on the direct conversion of CO2 to dimethyl ether in a fixed bed membrane reactor

Auteurs: Serena POTO, Fausto GALLUCCI, M. Fernanda NEIRA D’ANGELO
Publié dans: 26th International Symposium on Chemical Reaction Engineering (ISCRE-26), 2021
Éditeur: Department of Chemical Engineering Indian Institute of Technology Delhi

Techno-economic assessment of the dimethyl ether synthesis via CO2 hydrogenation:conventional vs membrane assisted process (poster)

Auteurs: Serena Poto, Thomas Vink, Fausto Gallucci, M. Fernanda Neira d’Angelo
Publié dans: Netherlands Process Symposium (NPS-17), 2022
Éditeur: NPS

Carbon molecular sieve membranes for water separation in CO2 hydrogenation reactions: effect of the carbonization temperature (oral)

Auteurs: Serena Poto, Alejo Aguirre, Margot A. Llosa Tanco, David A. Pacheco Tanaka, Fausto Gallucci, M. Fernanda Neira d’Angelo
Publié dans: Euromembrane 2022, 2022
Éditeur: EMS

In2O3 Nanoparticles for Electrocatalytic CO2 Reduction to Formate: effects of catalyst phase and GDE configuration (poster)

Auteurs: T. Wissink, M.C. Figueiredo, E.J.M. Hensen
Publié dans: Electrochemistry 2022 conference, 2022
Éditeur: Electrochemistry 2022 conference
DOI: 10.5281/zenodo.7846297

Design of membrane based gas-liquid absorption units: a fast, efficient, high throughput batch to continuous methodology

Auteurs: E. Ferreri, C. Castel, E. Favre
Publié dans: ECCE13 (13th European Congress of Chemical Engineering, 2021
Éditeur: DECHEMA e.V.

CO2 direct hydrogenation to DME via membrane reactor (oral)

Auteurs: Serena Poto, Margot A. Llosa Tanco, D.A. Pacheco Tanaka, F. Gallucci, M.F. Neira d'Angelo
Publié dans: C2Fuel workshop: International Workshop on CO2 capture and utilization, 2021
Éditeur: C2Fuel - TU/e

Electrochemical Reduction of CO2 to Formate on Indium and Bismuth Catalysts

Auteurs: Tim Wissink
Publié dans: 2023, ISBN 978-90-386-5880-3
Éditeur: Eindhoven University of Technology

One-step CO2 hydrogenation to dimethyl ether via packed bed membrane reactors

Auteurs: Serena Poto
Publié dans: 2023
Éditeur: Eindhoven University of Technology

Evaluation of the relevant mass and heat transfer phenomena in a packed bed membrane reactor for the direct conversion of CO2 to dimethyl ether

Auteurs: Serena Poto, Huub van den Bogaard, Fausto Gallucci , M. Fernanda Neira d’Angelo
Publié dans: Fuel 350 (2023) 128783, 2023, ISSN 0016-2361
Éditeur: Elsevier BV
DOI: 10.1016/j.fuel.2023.128783

Techno economic assessment of the one-step CO2 conversion to dimethyl ether: conventional vs membrane-assisted process

Auteurs: Serena Poto, Thomas Vink, Pierre Oliver, Fausto Gallucci, M. Fernanda Neira d’Angelo
Publié dans: Journal of CO2 Utilization Volume 69, March 2023, 102419, 2023, ISSN 2212-9820
Éditeur: Elsevier BV
DOI: 10.1016/j.jcou.2023.102419

Evolution of bismuth oxide catalysts during electrochemical CO2 reduction

Auteurs: Wissink, T.; Man, A.J.W.; Chen, W.; Heinrichs, J.M.J.J.; van de Poll, R. C. J.; Figueiredo, M. C.; Hensen, E. J. M
Publié dans: Journal of CO2 Utilization, 2023, Page(s) Volume 77, November 2023, 102604, ISSN 2212-9820
Éditeur: Elsevier BV
DOI: 10.1016/j.jcou.2023.102604

Kinetic modelling of the methanol synthesis from CO2 and H2 over a CuO/CeO2/ZrO2 catalyst: The role of CO2 and CO hydrogenation

Auteurs: Serena Poto, Damian Vico van Berkel, Fausto Gallucci, M. Fernanda Neira d’Angelo
Publié dans: Chemical Engineering Journal, 2022, ISSN 1385-8947
Éditeur: Elsevier BV
DOI: 10.1016/j.cej.2022.134946

Experimental investigation of a packed bed membrane reactor for the direct conversion of CO2 to dimethyl ether

Auteurs: Serena Poto, Margot Anabell Llosa-Tanco, David Alfredo Pacheco-Tanaka, Fausto Gallucci, M. Fernanda Neira d’Angelo
Publié dans: Journal of CO2 Utilization, 2023, Page(s) Volume 72, June 2023, 102513, ISSN 2212-9820
Éditeur: Elsevier BV
DOI: 10.1016/j.jcou.2023.102513

Stability of In2O3 Nanoparticles in PTFEcontaining Gas Diffusion Electrodes for CO2 electroreduction to Formate

Auteurs: Tim Wissink; Rim C.J. van de Poll; Marta C. Figueiredo; Emiel J.M. Hensen
Publié dans: Journal of CO2 Utilization Volume 67, January 2023, 102331, Numéro 12, 2023, ISSN 2212-9820
Éditeur: Elsevier BV
DOI: 10.1016/j.jcou.2022.102331

Direct conversion of CO2 to dimethyl ether in a fixed bed membrane reactor: Influence of membrane properties and process conditions

Auteurs: Poto Serena; Gallucci Fausto; Neira d'Angelo M.Fernanda
Publié dans: Fuel, Numéro 1, 2021, Page(s) Volume 302, 15 October 2021, 121080, ISSN 0016-2361
Éditeur: Elsevier BV
DOI: 10.1016/j.fuel.2021.121080

Carbon molecular sieve membranes for water separation in CO2 hydrogenation reactions: effect of the carbonization temperature

Auteurs: Serena Poto, A. Aguirre, F. Huigh, Margot Anabell Llosa-Tanco, David Alfredo Pacheco-Tanaka, Fausto Gallucci, M. Fernanda Neira d’Angelo
Publié dans: Journal of Membrane Science Volume 677, 5 July 2023, 121613, 2023, ISSN 2155-9589
Éditeur: Elsevier
DOI: 10.1016/j.memsci.2023.121613

Vapor/gas separation through carbon molecular sieve membranes: Experimental and theoretical investigation

Auteurs: Serena Poto; Joost G.H. Endepoel; Margot Anabell Llosa-Tanco; D.A. Pacheco-Tanaka; Fausto Gallucci; M. Fernanda Neira d'Angelo
Publié dans: International Journal of Hydrogen Energy, Numéro 3, 2021, ISSN 0360-3199
Éditeur: Pergamon Press Ltd.
DOI: 10.1016/j.ijhydene.2021.10.155

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