Unravelling the secrets of Cu-based catalysts for C-H activation

Publicaciones

Structural Elucidation, Aggregation, and Dynamic Behaviour of N,N,N,N-Copper(I) Schiff Base Complexes in Solid and in Solution: A Combined NMR, X-ray Spectroscopic and Crystallographic Investigation

Autores: Isabelle Gerz, Dr. Sergio Augusto Venturinelli Jannuzzi, Dr. Knut T. Hylland, Dr. Chiara Negri, Dr. David S. Wragg, Dr. Sigurd Øien-Ødegaard, Prof. Mats Tilset, Prof. Unni Olsbye, Prof. Serena DeBeer, Prof. Mohamed Amedjkouh
Publicado en: European Journal of Inorganic Chemistry, Edición 46, 2021, Página(s) 4762-4775, ISSN 1099-0682
Editor: Wiley-VCH GmbH
DOI: 10.1002/ejic.202100722

Modulation of [CuOH/O]+ Properties in [2,2′-Bipyridine]2 Homoleptic Complexes through Substitution at the 6,6’ Position by Methyl Groups

Autores: Alessandro Damin; Matteo Bonomo; Barbara Centrella; Matteo Signorile; Claudia Barolo; Silvia Bordiga
Publicado en: ACS Omega, Edición Volume 9, Edición 14, 2024, Página(s) 16610−16620, ISSN 2470-1343
Editor: American Chemical Society
DOI: 10.1021/acsomega.4c00598

Ancestral sequence reconstruction as a tool to study the evolution of wood decaying fungi

Autores: Iván Ayuso-Fernández; Gonzalo Molpeceres; Susana Camarero; Francisco Javier Ruiz-Dueñas; Angel T. Martínez
Publicado en: Frontiers in Fungal Biology, Edición Volume 3, article 1003489, 2022, ISSN 2673-6128
Editor: Frontiers Media S.A.
DOI: 10.3389/ffunb.2022.1003489

Combining Valence-to-Core X-ray Emission and Cu K-edge X-ray Absorption Spectroscopies to Experimentally Assess Oxidation State in Organometallic Cu(I)/(II)/(III) Complexes

Autores: Blaise L. Geoghegan; Yang Liu; Sergey Peredkov; Sebastian Dechert; Franc Meyer; Serena DeBeer; George E. Cutsail
Publicado en: Journal of the American Chemical Society, Edición Volume 144, issue 6, January 2022, 2022, Página(s) 2520–2534, ISSN 0002-7863
Editor: American Chemical Society
DOI: 10.1021/jacs.1c09505

Copper Pairing in the Mordenite Framework as a Function of the CuI/CuII Speciation

Autores: Gabriele Deplano, Dr. Andrea Martini, Dr. Matteo Signorile, Dr. Elisa Borfecchia, Dr. Valentina Crocellà, Prof. Stian Svelle, Prof. Silvia Bordiga
Publicado en: Angewandte Chemie, Edición 49, 2021, Página(s) 25891-25896, ISSN 1521-3757
Editor: Wiley-VCH GmbH
DOI: 10.1002/anie.202109705

Titration of Cu(I) Sites in Cu-ZSM-5 by Volumetric CO Adsorption

Autores: Gabriele Deplano, Matteo Signorile, Valentina Crocellà, Natale Gabriele Porcaro, Cesare Atzori, Bjørn Gading Solemsli, Stian Svelle, and Silvia Bordiga*
Publicado en: ACS Applied Materials & Interfaces, Edición Volume 14, Edición 18, April 2022, 2022, Página(s) 21059–21068, ISSN 1944-8244
Editor: American Chemical Society
DOI: 10.1021/acsami.2c03370

Reducibility of Cu-zeolites and stability of Cu+ monocarbonyl adducts: Qualitative and quantitative relationships from MCR-XAS and DFT

Autores: Gabriele Deplano; Matteo Signorile; Cesare Atzori; Davide Salusso; Elisa Borfecchia; Valentina Crocellà; Silvia Bordiga
Publicado en: Catalysis Today, Edición Volume 427, 114403,, 2023, ISSN 0920-5861
Editor: Elsevier BV
DOI: 10.1016/j.cattod.2023.114403

Investigating the role of Cu-oxo species in Cu-nitrate formation over Cu-CHA catalysts.

Autores: Chiara Negri; Andrea Martini; Gabriele Deplano; Kirill A. Lomachenko; Ton V. W. Janssens; Elisa Borfecchia; Gloria Berlier; Silvia Bordiga
Publicado en: Physical Chemistry Chemical Physics, Edición 23, 2021, Página(s) 18322-18337, ISSN 1463-9084
Editor: The Royal Society of Chemistry
DOI: 10.1039/d1cp01754c

Integrated Experimental and Theoretical Investigation of Copper Active Site Properties of a Lytic Polysaccharide Monooxygenase from Serratia marcescens

Autores: Alessia Munzone, Manon Pujol, Ashish Tamhankar, Chris Joseph, Ievgen Mazurenko, Marius Réglier, Sergio A. V. Jannuzzi, Antoine Royant, Giuseppe Sicoli, Serena DeBeer, Maylis Orio, A. Jalila Simaan, and Christophe Decroos
Publicado en: Inorganic Chemistry, Edición Volume 63, Edición 24, 2024, Página(s) 11063-11078, ISSN 0020-1669
Editor: American Chemical Society
DOI: 10.1021/acs.inorgchem.4c00602

Lytic polysaccharide monooxygenases: enzymes for controlled and site-specific Fenton-like chemistry

Autores: B. Bissaro & V.G.H. Eijsink
Publicado en: Essays in Biochemistry, Edición Mar 18;Volume 67, issue 3, March 2023, 2023, Página(s) 575-584, ISSN 0071-1365
Editor: Portland Press, Ltd.
DOI: 10.1042/ebc20220250

Reductants fuel lytic polysaccharide monooxygenase activity in a pH-dependent manner

Autores: Ole Golten, Iván Ayuso-Fernández, Kelsi R. Hall, Anton A. Stepnov, Morten Sørlie, Åsmund Kjendseth Røhr, Vincent G. H. Eijsink
Publicado en: FEBS Letters, Edición Volume 597, Edición 10, 2023, Página(s) 1363-1374, ISSN 0014-5793
Editor: Elsevier BV
DOI: 10.1002/1873-3468.14629

Understanding C–H activation in light alkanes over Cu-MOR zeolites by coupling advanced spectroscopy and temperature-programmed reduction experiments

Autores: Karoline Kvande; Beatrice Garetto; Gabriele Deplano; Matteo Signorile; Bjørn Gading Solemsli; Sebastian Prodinger; Unni Olsbye; Pablo Beato; Silvia Bordiga; Stian Svelle; Elisa Borfecchia
Publicado en: Chemical Science, Edición August 2023, volume 14, 2023, Página(s) 9704–9723, ISSN 2041-6520
Editor: Royal Society of Chemistry
DOI: 10.1039/d3sc01677c

A multi-technique approach to unveil the redox behaviour and potentiality of homoleptic CuI complexes based on substituted bipyridine ligands in oxygenation reactions

Autores: Barbara Centrella; Gabriele Deplano; Alessandro Damin; Matteo Signorile; Mariagrazia Tortora; Claudia Barolo; Matteo Bonomo; Silvia Bordiga
Publicado en: Dalton Transactions, Edición Edición 51, July 2022, 2022, Página(s) 14439-14451, ISSN 1477-9234
Editor: The Royal Society of Chemistry
DOI: 10.1039/d2dt01234k

Reactivity of methoxy species towards methylation and oligomerization in Cu-zeolite systems

Autores: Bjørn Gading Solemsli, Izar Capel Berdiell, Sebastian Prodinger, Karoline Kvande, Gabriele Deplano, Unni Olsbye, Pablo Beato, Silvia Bordiga, Stian Svelle
Publicado en: Catalysis Today, Edición Volume 436, Article 114729, 2024, ISSN 0920-5861
Editor: Elsevier BV
DOI: 10.1016/j.cattod.2024.114729

Towards a unified understanding of the copper sites in particulate methane monooxygenase: an X-ray absorption spectroscopic investigation

Autores: George E. Cutsail; Matthew O. Ross; Amy C. Rosenzweig; Serena DeBeer
Publicado en: Chemical Science, Edición 12, 2021, Página(s) 6194-6209, ISSN 2041-6539
Editor: The Royal Society of Chemistry
DOI: 10.1039/d1sc00676b

Assessing the Influence of Zeolite Composition on Oxygen-Bridged Diamino Dicopper(II) Complexes in Cu-CHA DeNOx Catalysts by Machine Learning-Assisted X-ray Absorption Spectroscopy

Autores: Andrea Martini; Chiara Negri; Luca Bugarin; Gabriele Deplano; Reza K. Abasabadi; Kirill A. Lomachenko; Ton V. W. Janssens; Silvia Bordiga; Gloria Berlier; Elisa Borfecchia
Publicado en: The Journal of Physical Chemistry Letters, Edición Volume 13, Edición 26, July 2022, 2022, Página(s) 6164-6170, ISSN 1948-7185
Editor: American Chemical Society
DOI: 10.1021/acs.jpclett.2c01107

Visible light-exposed lignin facilitates cellulose solubilization by lytic polysaccharide monooxygenases

Autores: Eirik G. Kommedal; Camilla F. Angeltveit; Leesa J. Klau; Iván Ayuso-Fernández; Bjørnar Arstad; Simen G. Antonsen; Yngve Stenstrøm; Dag Ekeberg; Francisco Gírio; Florbela Carvalheiro; Svein J. Horn; Finn Lillelund Aachmann; Vincent G. H. Eijsink
Publicado en: Nature Communications, Edición Volume 14, article 1063, 2023, 2023, Página(s) 1-12, ISSN 2041-1723
Editor: Nature Publishing Group
DOI: 10.1038/s41467-023-36660-4

Influence of ion mobility on the redox and catalytic properties of Cu ions in zeolites

Autores: Signorile, Matteo; Borfecchia, Elisa; Bordiga, Silvia; Berlier, Gloria
Publicado en: Chemical Science, Edición Edición 35, August 2022, 2022, Página(s) 10238-10250, ISSN 2041-6520
Editor: Royal Society of Chemistry
DOI: 10.1039/d2sc03565k

Investigating the role of aromatic core residues in protecting against oxidative damage in lytic polysaccharide monooxygenase SmAA10A

Autores: Moe, Trond
Publicado en: 2022
Editor: NMBU

The Impact of a Structurally Conserved Second Sphere Residue in Lytic Polysaccharide Monooxygenase Catalysis

Autores: Skaali, Rannei
Publicado en: 2022
Editor: NMBU

The roles of conserved second sphere residues in lytic polysaccharide monooxygenase catalysis

Autores: Mollatt, Maja
Publicado en: 2022
Editor: NMBU

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