Unravelling the secrets of Cu-based catalysts for C-H activation

Publikacje

Structural Elucidation, Aggregation, and Dynamic Behaviour of N,N,N,N-Copper(I) Schiff Base Complexes in Solid and in Solution: A Combined NMR, X-ray Spectroscopic and Crystallographic Investigation

Autorzy: Isabelle Gerz, Dr. Sergio Augusto Venturinelli Jannuzzi, Dr. Knut T. Hylland, Dr. Chiara Negri, Dr. David S. Wragg, Dr. Sigurd Øien-Ødegaard, Prof. Mats Tilset, Prof. Unni Olsbye, Prof. Serena DeBeer, Prof. Mohamed Amedjkouh
Opublikowane w: European Journal of Inorganic Chemistry, Numer 46, 2021, Strona(/y) 4762-4775, ISSN 1099-0682
Wydawca: Wiley-VCH GmbH
DOI: 10.1002/ejic.202100722

Modulation of [CuOH/O]+ Properties in [2,2′-Bipyridine]2 Homoleptic Complexes through Substitution at the 6,6’ Position by Methyl Groups

Autorzy: Alessandro Damin; Matteo Bonomo; Barbara Centrella; Matteo Signorile; Claudia Barolo; Silvia Bordiga
Opublikowane w: ACS Omega, Numer Volume 9, Numer 14, 2024, Strona(/y) 16610−16620, ISSN 2470-1343
Wydawca: American Chemical Society
DOI: 10.1021/acsomega.4c00598

Ancestral sequence reconstruction as a tool to study the evolution of wood decaying fungi

Autorzy: Iván Ayuso-Fernández; Gonzalo Molpeceres; Susana Camarero; Francisco Javier Ruiz-Dueñas; Angel T. Martínez
Opublikowane w: Frontiers in Fungal Biology, Numer Volume 3, article 1003489, 2022, ISSN 2673-6128
Wydawca: Frontiers Media S.A.
DOI: 10.3389/ffunb.2022.1003489

Combining Valence-to-Core X-ray Emission and Cu K-edge X-ray Absorption Spectroscopies to Experimentally Assess Oxidation State in Organometallic Cu(I)/(II)/(III) Complexes

Autorzy: Blaise L. Geoghegan; Yang Liu; Sergey Peredkov; Sebastian Dechert; Franc Meyer; Serena DeBeer; George E. Cutsail
Opublikowane w: Journal of the American Chemical Society, Numer Volume 144, issue 6, January 2022, 2022, Strona(/y) 2520–2534, ISSN 0002-7863
Wydawca: American Chemical Society
DOI: 10.1021/jacs.1c09505

Copper Pairing in the Mordenite Framework as a Function of the CuI/CuII Speciation

Autorzy: Gabriele Deplano, Dr. Andrea Martini, Dr. Matteo Signorile, Dr. Elisa Borfecchia, Dr. Valentina Crocellà, Prof. Stian Svelle, Prof. Silvia Bordiga
Opublikowane w: Angewandte Chemie, Numer 49, 2021, Strona(/y) 25891-25896, ISSN 1521-3757
Wydawca: Wiley-VCH GmbH
DOI: 10.1002/anie.202109705

Titration of Cu(I) Sites in Cu-ZSM-5 by Volumetric CO Adsorption

Autorzy: Gabriele Deplano, Matteo Signorile, Valentina Crocellà, Natale Gabriele Porcaro, Cesare Atzori, Bjørn Gading Solemsli, Stian Svelle, and Silvia Bordiga*
Opublikowane w: ACS Applied Materials & Interfaces, Numer Volume 14, Numer 18, April 2022, 2022, Strona(/y) 21059–21068, ISSN 1944-8244
Wydawca: American Chemical Society
DOI: 10.1021/acsami.2c03370

Reducibility of Cu-zeolites and stability of Cu+ monocarbonyl adducts: Qualitative and quantitative relationships from MCR-XAS and DFT

Autorzy: Gabriele Deplano; Matteo Signorile; Cesare Atzori; Davide Salusso; Elisa Borfecchia; Valentina Crocellà; Silvia Bordiga
Opublikowane w: Catalysis Today, Numer Volume 427, 114403,, 2023, ISSN 0920-5861
Wydawca: Elsevier BV
DOI: 10.1016/j.cattod.2023.114403

Investigating the role of Cu-oxo species in Cu-nitrate formation over Cu-CHA catalysts.

Autorzy: Chiara Negri; Andrea Martini; Gabriele Deplano; Kirill A. Lomachenko; Ton V. W. Janssens; Elisa Borfecchia; Gloria Berlier; Silvia Bordiga
Opublikowane w: Physical Chemistry Chemical Physics, Numer 23, 2021, Strona(/y) 18322-18337, ISSN 1463-9084
Wydawca: The Royal Society of Chemistry
DOI: 10.1039/d1cp01754c

Integrated Experimental and Theoretical Investigation of Copper Active Site Properties of a Lytic Polysaccharide Monooxygenase from Serratia marcescens

Autorzy: Alessia Munzone, Manon Pujol, Ashish Tamhankar, Chris Joseph, Ievgen Mazurenko, Marius Réglier, Sergio A. V. Jannuzzi, Antoine Royant, Giuseppe Sicoli, Serena DeBeer, Maylis Orio, A. Jalila Simaan, and Christophe Decroos
Opublikowane w: Inorganic Chemistry, Numer Volume 63, Numer 24, 2024, Strona(/y) 11063-11078, ISSN 0020-1669
Wydawca: American Chemical Society
DOI: 10.1021/acs.inorgchem.4c00602

Lytic polysaccharide monooxygenases: enzymes for controlled and site-specific Fenton-like chemistry

Autorzy: B. Bissaro & V.G.H. Eijsink
Opublikowane w: Essays in Biochemistry, Numer Mar 18;Volume 67, issue 3, March 2023, 2023, Strona(/y) 575-584, ISSN 0071-1365
Wydawca: Portland Press, Ltd.
DOI: 10.1042/ebc20220250

Reductants fuel lytic polysaccharide monooxygenase activity in a pH-dependent manner

Autorzy: Ole Golten, Iván Ayuso-Fernández, Kelsi R. Hall, Anton A. Stepnov, Morten Sørlie, Åsmund Kjendseth Røhr, Vincent G. H. Eijsink
Opublikowane w: FEBS Letters, Numer Volume 597, Numer 10, 2023, Strona(/y) 1363-1374, ISSN 0014-5793
Wydawca: Elsevier BV
DOI: 10.1002/1873-3468.14629

Understanding C–H activation in light alkanes over Cu-MOR zeolites by coupling advanced spectroscopy and temperature-programmed reduction experiments

Autorzy: Karoline Kvande; Beatrice Garetto; Gabriele Deplano; Matteo Signorile; Bjørn Gading Solemsli; Sebastian Prodinger; Unni Olsbye; Pablo Beato; Silvia Bordiga; Stian Svelle; Elisa Borfecchia
Opublikowane w: Chemical Science, Numer August 2023, volume 14, 2023, Strona(/y) 9704–9723, ISSN 2041-6520
Wydawca: Royal Society of Chemistry
DOI: 10.1039/d3sc01677c

A multi-technique approach to unveil the redox behaviour and potentiality of homoleptic CuI complexes based on substituted bipyridine ligands in oxygenation reactions

Autorzy: Barbara Centrella; Gabriele Deplano; Alessandro Damin; Matteo Signorile; Mariagrazia Tortora; Claudia Barolo; Matteo Bonomo; Silvia Bordiga
Opublikowane w: Dalton Transactions, Numer Numer 51, July 2022, 2022, Strona(/y) 14439-14451, ISSN 1477-9234
Wydawca: The Royal Society of Chemistry
DOI: 10.1039/d2dt01234k

Reactivity of methoxy species towards methylation and oligomerization in Cu-zeolite systems

Autorzy: Bjørn Gading Solemsli, Izar Capel Berdiell, Sebastian Prodinger, Karoline Kvande, Gabriele Deplano, Unni Olsbye, Pablo Beato, Silvia Bordiga, Stian Svelle
Opublikowane w: Catalysis Today, Numer Volume 436, Article 114729, 2024, ISSN 0920-5861
Wydawca: Elsevier BV
DOI: 10.1016/j.cattod.2024.114729

Towards a unified understanding of the copper sites in particulate methane monooxygenase: an X-ray absorption spectroscopic investigation

Autorzy: George E. Cutsail; Matthew O. Ross; Amy C. Rosenzweig; Serena DeBeer
Opublikowane w: Chemical Science, Numer 12, 2021, Strona(/y) 6194-6209, ISSN 2041-6539
Wydawca: The Royal Society of Chemistry
DOI: 10.1039/d1sc00676b

Assessing the Influence of Zeolite Composition on Oxygen-Bridged Diamino Dicopper(II) Complexes in Cu-CHA DeNOx Catalysts by Machine Learning-Assisted X-ray Absorption Spectroscopy

Autorzy: Andrea Martini; Chiara Negri; Luca Bugarin; Gabriele Deplano; Reza K. Abasabadi; Kirill A. Lomachenko; Ton V. W. Janssens; Silvia Bordiga; Gloria Berlier; Elisa Borfecchia
Opublikowane w: The Journal of Physical Chemistry Letters, Numer Volume 13, Numer 26, July 2022, 2022, Strona(/y) 6164-6170, ISSN 1948-7185
Wydawca: American Chemical Society
DOI: 10.1021/acs.jpclett.2c01107

Visible light-exposed lignin facilitates cellulose solubilization by lytic polysaccharide monooxygenases

Autorzy: Eirik G. Kommedal; Camilla F. Angeltveit; Leesa J. Klau; Iván Ayuso-Fernández; Bjørnar Arstad; Simen G. Antonsen; Yngve Stenstrøm; Dag Ekeberg; Francisco Gírio; Florbela Carvalheiro; Svein J. Horn; Finn Lillelund Aachmann; Vincent G. H. Eijsink
Opublikowane w: Nature Communications, Numer Volume 14, article 1063, 2023, 2023, Strona(/y) 1-12, ISSN 2041-1723
Wydawca: Nature Publishing Group
DOI: 10.1038/s41467-023-36660-4

Influence of ion mobility on the redox and catalytic properties of Cu ions in zeolites

Autorzy: Signorile, Matteo; Borfecchia, Elisa; Bordiga, Silvia; Berlier, Gloria
Opublikowane w: Chemical Science, Numer Numer 35, August 2022, 2022, Strona(/y) 10238-10250, ISSN 2041-6520
Wydawca: Royal Society of Chemistry
DOI: 10.1039/d2sc03565k

Investigating the role of aromatic core residues in protecting against oxidative damage in lytic polysaccharide monooxygenase SmAA10A

Autorzy: Moe, Trond
Opublikowane w: 2022
Wydawca: NMBU

The Impact of a Structurally Conserved Second Sphere Residue in Lytic Polysaccharide Monooxygenase Catalysis

Autorzy: Skaali, Rannei
Opublikowane w: 2022
Wydawca: NMBU

The roles of conserved second sphere residues in lytic polysaccharide monooxygenase catalysis

Autorzy: Mollatt, Maja
Opublikowane w: 2022
Wydawca: NMBU

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