Unravelling the secrets of Cu-based catalysts for C-H activation

Publications

Structural Elucidation, Aggregation, and Dynamic Behaviour of N,N,N,N-Copper(I) Schiff Base Complexes in Solid and in Solution: A Combined NMR, X-ray Spectroscopic and Crystallographic Investigation

Author(s): Isabelle Gerz, Dr. Sergio Augusto Venturinelli Jannuzzi, Dr. Knut T. Hylland, Dr. Chiara Negri, Dr. David S. Wragg, Dr. Sigurd Øien-Ødegaard, Prof. Mats Tilset, Prof. Unni Olsbye, Prof. Serena DeBeer, Prof. Mohamed Amedjkouh
Published in: European Journal of Inorganic Chemistry, Issue 46, 2021, Page(s) 4762-4775, ISSN 1099-0682
Publisher: Wiley-VCH GmbH
DOI: 10.1002/ejic.202100722

Modulation of [CuOH/O]+ Properties in [2,2′-Bipyridine]2 Homoleptic Complexes through Substitution at the 6,6’ Position by Methyl Groups

Author(s): Alessandro Damin; Matteo Bonomo; Barbara Centrella; Matteo Signorile; Claudia Barolo; Silvia Bordiga
Published in: ACS Omega, Issue Volume 9, Issue 14, 2024, Page(s) 16610−16620, ISSN 2470-1343
Publisher: American Chemical Society
DOI: 10.1021/acsomega.4c00598

Ancestral sequence reconstruction as a tool to study the evolution of wood decaying fungi

Author(s): Iván Ayuso-Fernández; Gonzalo Molpeceres; Susana Camarero; Francisco Javier Ruiz-Dueñas; Angel T. Martínez
Published in: Frontiers in Fungal Biology, Issue Volume 3, article 1003489, 2022, ISSN 2673-6128
Publisher: Frontiers Media S.A.
DOI: 10.3389/ffunb.2022.1003489

Combining Valence-to-Core X-ray Emission and Cu K-edge X-ray Absorption Spectroscopies to Experimentally Assess Oxidation State in Organometallic Cu(I)/(II)/(III) Complexes

Author(s): Blaise L. Geoghegan; Yang Liu; Sergey Peredkov; Sebastian Dechert; Franc Meyer; Serena DeBeer; George E. Cutsail
Published in: Journal of the American Chemical Society, Issue Volume 144, issue 6, January 2022, 2022, Page(s) 2520–2534, ISSN 0002-7863
Publisher: American Chemical Society
DOI: 10.1021/jacs.1c09505

Copper Pairing in the Mordenite Framework as a Function of the CuI/CuII Speciation

Author(s): Gabriele Deplano, Dr. Andrea Martini, Dr. Matteo Signorile, Dr. Elisa Borfecchia, Dr. Valentina Crocellà, Prof. Stian Svelle, Prof. Silvia Bordiga
Published in: Angewandte Chemie, Issue 49, 2021, Page(s) 25891-25896, ISSN 1521-3757
Publisher: Wiley-VCH GmbH
DOI: 10.1002/anie.202109705

Titration of Cu(I) Sites in Cu-ZSM-5 by Volumetric CO Adsorption

Author(s): Gabriele Deplano, Matteo Signorile, Valentina Crocellà, Natale Gabriele Porcaro, Cesare Atzori, Bjørn Gading Solemsli, Stian Svelle, and Silvia Bordiga*
Published in: ACS Applied Materials & Interfaces, Issue Volume 14, Issue 18, April 2022, 2022, Page(s) 21059–21068, ISSN 1944-8244
Publisher: American Chemical Society
DOI: 10.1021/acsami.2c03370

Reducibility of Cu-zeolites and stability of Cu+ monocarbonyl adducts: Qualitative and quantitative relationships from MCR-XAS and DFT

Author(s): Gabriele Deplano; Matteo Signorile; Cesare Atzori; Davide Salusso; Elisa Borfecchia; Valentina Crocellà; Silvia Bordiga
Published in: Catalysis Today, Issue Volume 427, 114403,, 2023, ISSN 0920-5861
Publisher: Elsevier BV
DOI: 10.1016/j.cattod.2023.114403

Investigating the role of Cu-oxo species in Cu-nitrate formation over Cu-CHA catalysts.

Author(s): Chiara Negri; Andrea Martini; Gabriele Deplano; Kirill A. Lomachenko; Ton V. W. Janssens; Elisa Borfecchia; Gloria Berlier; Silvia Bordiga
Published in: Physical Chemistry Chemical Physics, Issue 23, 2021, Page(s) 18322-18337, ISSN 1463-9084
Publisher: The Royal Society of Chemistry
DOI: 10.1039/d1cp01754c

Integrated Experimental and Theoretical Investigation of Copper Active Site Properties of a Lytic Polysaccharide Monooxygenase from Serratia marcescens

Author(s): Alessia Munzone, Manon Pujol, Ashish Tamhankar, Chris Joseph, Ievgen Mazurenko, Marius Réglier, Sergio A. V. Jannuzzi, Antoine Royant, Giuseppe Sicoli, Serena DeBeer, Maylis Orio, A. Jalila Simaan, and Christophe Decroos
Published in: Inorganic Chemistry, Issue Volume 63, Issue 24, 2024, Page(s) 11063-11078, ISSN 0020-1669
Publisher: American Chemical Society
DOI: 10.1021/acs.inorgchem.4c00602

Lytic polysaccharide monooxygenases: enzymes for controlled and site-specific Fenton-like chemistry

Author(s): B. Bissaro & V.G.H. Eijsink
Published in: Essays in Biochemistry, Issue Mar 18;Volume 67, issue 3, March 2023, 2023, Page(s) 575-584, ISSN 0071-1365
Publisher: Portland Press, Ltd.
DOI: 10.1042/ebc20220250

Reductants fuel lytic polysaccharide monooxygenase activity in a pH-dependent manner

Author(s): Ole Golten, Iván Ayuso-Fernández, Kelsi R. Hall, Anton A. Stepnov, Morten Sørlie, Åsmund Kjendseth Røhr, Vincent G. H. Eijsink
Published in: FEBS Letters, Issue Volume 597, Issue 10, 2023, Page(s) 1363-1374, ISSN 0014-5793
Publisher: Elsevier BV
DOI: 10.1002/1873-3468.14629

Understanding C–H activation in light alkanes over Cu-MOR zeolites by coupling advanced spectroscopy and temperature-programmed reduction experiments

Author(s): Karoline Kvande; Beatrice Garetto; Gabriele Deplano; Matteo Signorile; Bjørn Gading Solemsli; Sebastian Prodinger; Unni Olsbye; Pablo Beato; Silvia Bordiga; Stian Svelle; Elisa Borfecchia
Published in: Chemical Science, Issue August 2023, volume 14, 2023, Page(s) 9704–9723, ISSN 2041-6520
Publisher: Royal Society of Chemistry
DOI: 10.1039/d3sc01677c

A multi-technique approach to unveil the redox behaviour and potentiality of homoleptic CuI complexes based on substituted bipyridine ligands in oxygenation reactions

Author(s): Barbara Centrella; Gabriele Deplano; Alessandro Damin; Matteo Signorile; Mariagrazia Tortora; Claudia Barolo; Matteo Bonomo; Silvia Bordiga
Published in: Dalton Transactions, Issue Issue 51, July 2022, 2022, Page(s) 14439-14451, ISSN 1477-9234
Publisher: The Royal Society of Chemistry
DOI: 10.1039/d2dt01234k

Reactivity of methoxy species towards methylation and oligomerization in Cu-zeolite systems

Author(s): Bjørn Gading Solemsli, Izar Capel Berdiell, Sebastian Prodinger, Karoline Kvande, Gabriele Deplano, Unni Olsbye, Pablo Beato, Silvia Bordiga, Stian Svelle
Published in: Catalysis Today, Issue Volume 436, Article 114729, 2024, ISSN 0920-5861
Publisher: Elsevier BV
DOI: 10.1016/j.cattod.2024.114729

Towards a unified understanding of the copper sites in particulate methane monooxygenase: an X-ray absorption spectroscopic investigation

Author(s): George E. Cutsail; Matthew O. Ross; Amy C. Rosenzweig; Serena DeBeer
Published in: Chemical Science, Issue 12, 2021, Page(s) 6194-6209, ISSN 2041-6539
Publisher: The Royal Society of Chemistry
DOI: 10.1039/d1sc00676b

Assessing the Influence of Zeolite Composition on Oxygen-Bridged Diamino Dicopper(II) Complexes in Cu-CHA DeNOx Catalysts by Machine Learning-Assisted X-ray Absorption Spectroscopy

Author(s): Andrea Martini; Chiara Negri; Luca Bugarin; Gabriele Deplano; Reza K. Abasabadi; Kirill A. Lomachenko; Ton V. W. Janssens; Silvia Bordiga; Gloria Berlier; Elisa Borfecchia
Published in: The Journal of Physical Chemistry Letters, Issue Volume 13, Issue 26, July 2022, 2022, Page(s) 6164-6170, ISSN 1948-7185
Publisher: American Chemical Society
DOI: 10.1021/acs.jpclett.2c01107

Visible light-exposed lignin facilitates cellulose solubilization by lytic polysaccharide monooxygenases

Author(s): Eirik G. Kommedal; Camilla F. Angeltveit; Leesa J. Klau; Iván Ayuso-Fernández; Bjørnar Arstad; Simen G. Antonsen; Yngve Stenstrøm; Dag Ekeberg; Francisco Gírio; Florbela Carvalheiro; Svein J. Horn; Finn Lillelund Aachmann; Vincent G. H. Eijsink
Published in: Nature Communications, Issue Volume 14, article 1063, 2023, 2023, Page(s) 1-12, ISSN 2041-1723
Publisher: Nature Publishing Group
DOI: 10.1038/s41467-023-36660-4

Influence of ion mobility on the redox and catalytic properties of Cu ions in zeolites

Author(s): Signorile, Matteo; Borfecchia, Elisa; Bordiga, Silvia; Berlier, Gloria
Published in: Chemical Science, Issue Issue 35, August 2022, 2022, Page(s) 10238-10250, ISSN 2041-6520
Publisher: Royal Society of Chemistry
DOI: 10.1039/d2sc03565k

Investigating the role of aromatic core residues in protecting against oxidative damage in lytic polysaccharide monooxygenase SmAA10A

Author(s): Moe, Trond
Published in: 2022
Publisher: NMBU

The Impact of a Structurally Conserved Second Sphere Residue in Lytic Polysaccharide Monooxygenase Catalysis

Author(s): Skaali, Rannei
Published in: 2022
Publisher: NMBU

The roles of conserved second sphere residues in lytic polysaccharide monooxygenase catalysis

Author(s): Mollatt, Maja
Published in: 2022
Publisher: NMBU

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