Unravelling the secrets of Cu-based catalysts for C-H activation

Publications

Structural Elucidation, Aggregation, and Dynamic Behaviour of N,N,N,N-Copper(I) Schiff Base Complexes in Solid and in Solution: A Combined NMR, X-ray Spectroscopic and Crystallographic Investigation

Auteurs: Isabelle Gerz, Dr. Sergio Augusto Venturinelli Jannuzzi, Dr. Knut T. Hylland, Dr. Chiara Negri, Dr. David S. Wragg, Dr. Sigurd Øien-Ødegaard, Prof. Mats Tilset, Prof. Unni Olsbye, Prof. Serena DeBeer, Prof. Mohamed Amedjkouh
Publié dans: European Journal of Inorganic Chemistry, Numéro 46, 2021, Page(s) 4762-4775, ISSN 1099-0682
Éditeur: Wiley-VCH GmbH
DOI: 10.1002/ejic.202100722

Modulation of [CuOH/O]+ Properties in [2,2′-Bipyridine]2 Homoleptic Complexes through Substitution at the 6,6’ Position by Methyl Groups

Auteurs: Alessandro Damin; Matteo Bonomo; Barbara Centrella; Matteo Signorile; Claudia Barolo; Silvia Bordiga
Publié dans: ACS Omega, Numéro Volume 9, Numéro 14, 2024, Page(s) 16610−16620, ISSN 2470-1343
Éditeur: American Chemical Society
DOI: 10.1021/acsomega.4c00598

Ancestral sequence reconstruction as a tool to study the evolution of wood decaying fungi

Auteurs: Iván Ayuso-Fernández; Gonzalo Molpeceres; Susana Camarero; Francisco Javier Ruiz-Dueñas; Angel T. Martínez
Publié dans: Frontiers in Fungal Biology, Numéro Volume 3, article 1003489, 2022, ISSN 2673-6128
Éditeur: Frontiers Media S.A.
DOI: 10.3389/ffunb.2022.1003489

Combining Valence-to-Core X-ray Emission and Cu K-edge X-ray Absorption Spectroscopies to Experimentally Assess Oxidation State in Organometallic Cu(I)/(II)/(III) Complexes

Auteurs: Blaise L. Geoghegan; Yang Liu; Sergey Peredkov; Sebastian Dechert; Franc Meyer; Serena DeBeer; George E. Cutsail
Publié dans: Journal of the American Chemical Society, Numéro Volume 144, issue 6, January 2022, 2022, Page(s) 2520–2534, ISSN 0002-7863
Éditeur: American Chemical Society
DOI: 10.1021/jacs.1c09505

Copper Pairing in the Mordenite Framework as a Function of the CuI/CuII Speciation

Auteurs: Gabriele Deplano, Dr. Andrea Martini, Dr. Matteo Signorile, Dr. Elisa Borfecchia, Dr. Valentina Crocellà, Prof. Stian Svelle, Prof. Silvia Bordiga
Publié dans: Angewandte Chemie, Numéro 49, 2021, Page(s) 25891-25896, ISSN 1521-3757
Éditeur: Wiley-VCH GmbH
DOI: 10.1002/anie.202109705

Titration of Cu(I) Sites in Cu-ZSM-5 by Volumetric CO Adsorption

Auteurs: Gabriele Deplano, Matteo Signorile, Valentina Crocellà, Natale Gabriele Porcaro, Cesare Atzori, Bjørn Gading Solemsli, Stian Svelle, and Silvia Bordiga*
Publié dans: ACS Applied Materials & Interfaces, Numéro Volume 14, Numéro 18, April 2022, 2022, Page(s) 21059–21068, ISSN 1944-8244
Éditeur: American Chemical Society
DOI: 10.1021/acsami.2c03370

Reducibility of Cu-zeolites and stability of Cu+ monocarbonyl adducts: Qualitative and quantitative relationships from MCR-XAS and DFT

Auteurs: Gabriele Deplano; Matteo Signorile; Cesare Atzori; Davide Salusso; Elisa Borfecchia; Valentina Crocellà; Silvia Bordiga
Publié dans: Catalysis Today, Numéro Volume 427, 114403,, 2023, ISSN 0920-5861
Éditeur: Elsevier BV
DOI: 10.1016/j.cattod.2023.114403

Investigating the role of Cu-oxo species in Cu-nitrate formation over Cu-CHA catalysts.

Auteurs: Chiara Negri; Andrea Martini; Gabriele Deplano; Kirill A. Lomachenko; Ton V. W. Janssens; Elisa Borfecchia; Gloria Berlier; Silvia Bordiga
Publié dans: Physical Chemistry Chemical Physics, Numéro 23, 2021, Page(s) 18322-18337, ISSN 1463-9084
Éditeur: The Royal Society of Chemistry
DOI: 10.1039/d1cp01754c

Integrated Experimental and Theoretical Investigation of Copper Active Site Properties of a Lytic Polysaccharide Monooxygenase from Serratia marcescens

Auteurs: Alessia Munzone, Manon Pujol, Ashish Tamhankar, Chris Joseph, Ievgen Mazurenko, Marius Réglier, Sergio A. V. Jannuzzi, Antoine Royant, Giuseppe Sicoli, Serena DeBeer, Maylis Orio, A. Jalila Simaan, and Christophe Decroos
Publié dans: Inorganic Chemistry, Numéro Volume 63, Numéro 24, 2024, Page(s) 11063-11078, ISSN 0020-1669
Éditeur: American Chemical Society
DOI: 10.1021/acs.inorgchem.4c00602

Lytic polysaccharide monooxygenases: enzymes for controlled and site-specific Fenton-like chemistry

Auteurs: B. Bissaro & V.G.H. Eijsink
Publié dans: Essays in Biochemistry, Numéro Mar 18;Volume 67, issue 3, March 2023, 2023, Page(s) 575-584, ISSN 0071-1365
Éditeur: Portland Press, Ltd.
DOI: 10.1042/ebc20220250

Reductants fuel lytic polysaccharide monooxygenase activity in a pH-dependent manner

Auteurs: Ole Golten, Iván Ayuso-Fernández, Kelsi R. Hall, Anton A. Stepnov, Morten Sørlie, Åsmund Kjendseth Røhr, Vincent G. H. Eijsink
Publié dans: FEBS Letters, Numéro Volume 597, Numéro 10, 2023, Page(s) 1363-1374, ISSN 0014-5793
Éditeur: Elsevier BV
DOI: 10.1002/1873-3468.14629

Understanding C–H activation in light alkanes over Cu-MOR zeolites by coupling advanced spectroscopy and temperature-programmed reduction experiments

Auteurs: Karoline Kvande; Beatrice Garetto; Gabriele Deplano; Matteo Signorile; Bjørn Gading Solemsli; Sebastian Prodinger; Unni Olsbye; Pablo Beato; Silvia Bordiga; Stian Svelle; Elisa Borfecchia
Publié dans: Chemical Science, Numéro August 2023, volume 14, 2023, Page(s) 9704–9723, ISSN 2041-6520
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d3sc01677c

A multi-technique approach to unveil the redox behaviour and potentiality of homoleptic CuI complexes based on substituted bipyridine ligands in oxygenation reactions

Auteurs: Barbara Centrella; Gabriele Deplano; Alessandro Damin; Matteo Signorile; Mariagrazia Tortora; Claudia Barolo; Matteo Bonomo; Silvia Bordiga
Publié dans: Dalton Transactions, Numéro Numéro 51, July 2022, 2022, Page(s) 14439-14451, ISSN 1477-9234
Éditeur: The Royal Society of Chemistry
DOI: 10.1039/d2dt01234k

Reactivity of methoxy species towards methylation and oligomerization in Cu-zeolite systems

Auteurs: Bjørn Gading Solemsli, Izar Capel Berdiell, Sebastian Prodinger, Karoline Kvande, Gabriele Deplano, Unni Olsbye, Pablo Beato, Silvia Bordiga, Stian Svelle
Publié dans: Catalysis Today, Numéro Volume 436, Article 114729, 2024, ISSN 0920-5861
Éditeur: Elsevier BV
DOI: 10.1016/j.cattod.2024.114729

Towards a unified understanding of the copper sites in particulate methane monooxygenase: an X-ray absorption spectroscopic investigation

Auteurs: George E. Cutsail; Matthew O. Ross; Amy C. Rosenzweig; Serena DeBeer
Publié dans: Chemical Science, Numéro 12, 2021, Page(s) 6194-6209, ISSN 2041-6539
Éditeur: The Royal Society of Chemistry
DOI: 10.1039/d1sc00676b

Assessing the Influence of Zeolite Composition on Oxygen-Bridged Diamino Dicopper(II) Complexes in Cu-CHA DeNOx Catalysts by Machine Learning-Assisted X-ray Absorption Spectroscopy

Auteurs: Andrea Martini; Chiara Negri; Luca Bugarin; Gabriele Deplano; Reza K. Abasabadi; Kirill A. Lomachenko; Ton V. W. Janssens; Silvia Bordiga; Gloria Berlier; Elisa Borfecchia
Publié dans: The Journal of Physical Chemistry Letters, Numéro Volume 13, Numéro 26, July 2022, 2022, Page(s) 6164-6170, ISSN 1948-7185
Éditeur: American Chemical Society
DOI: 10.1021/acs.jpclett.2c01107

Visible light-exposed lignin facilitates cellulose solubilization by lytic polysaccharide monooxygenases

Auteurs: Eirik G. Kommedal; Camilla F. Angeltveit; Leesa J. Klau; Iván Ayuso-Fernández; Bjørnar Arstad; Simen G. Antonsen; Yngve Stenstrøm; Dag Ekeberg; Francisco Gírio; Florbela Carvalheiro; Svein J. Horn; Finn Lillelund Aachmann; Vincent G. H. Eijsink
Publié dans: Nature Communications, Numéro Volume 14, article 1063, 2023, 2023, Page(s) 1-12, ISSN 2041-1723
Éditeur: Nature Publishing Group
DOI: 10.1038/s41467-023-36660-4

Influence of ion mobility on the redox and catalytic properties of Cu ions in zeolites

Auteurs: Signorile, Matteo; Borfecchia, Elisa; Bordiga, Silvia; Berlier, Gloria
Publié dans: Chemical Science, Numéro Numéro 35, August 2022, 2022, Page(s) 10238-10250, ISSN 2041-6520
Éditeur: Royal Society of Chemistry
DOI: 10.1039/d2sc03565k

Investigating the role of aromatic core residues in protecting against oxidative damage in lytic polysaccharide monooxygenase SmAA10A

Auteurs: Moe, Trond
Publié dans: 2022
Éditeur: NMBU

The Impact of a Structurally Conserved Second Sphere Residue in Lytic Polysaccharide Monooxygenase Catalysis

Auteurs: Skaali, Rannei
Publié dans: 2022
Éditeur: NMBU

The roles of conserved second sphere residues in lytic polysaccharide monooxygenase catalysis

Auteurs: Mollatt, Maja
Publié dans: 2022
Éditeur: NMBU

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