The project combined material development, connection design, structural testing, and numerical modelling to establish the proposed CCU composite concept. On the material side, strain-hardening magnesia-based cementitious composites were developed and assessed under CO2 curing, including component-scale slab fabrication and depth-resolved characterization of carbonation penetration, strength development, phase assemblage, microstructure, and CO2 uptake. On the connection side, a novel bolt–wedge demountable connection was designed and validated through push-out tests under different wedge slope ratios, bolt pretension levels, surface conditions, and loading protocols, supported by finite-element modelling and analytical interpretation. These two research lines were then brought together in prefabricated steel–SHMC push-out specimens to investigate how carbonation-induced material gradients affect interface shear behavior in reusable steel–cementitious assemblies.
The project achieved its main technical objectives. The developed SHMC system exceeded the target compressive strength of 50 MPa after CO2 curing, and the natural-fibre-reinforced slab reached a one-way carbonation depth of about 65 mm. The bolt–wedge connection improved slip resistance by converting bolt pretension into enhanced interface compression, and its behavior was captured through experiments, finite-element modelling, and a closed-form analytical model. At the structural level, the steel–SHMC studies showed that carbonation-induced through-thickness gradients strongly influence load transfer, stiffness evolution, and damage development at the interface. Compared with steel–C50 reference specimens, the steel–SHMC interfaces provided lower peak shear resistance but much greater deformation capacity and energy absorption, while also offering substantial CO2 uptake potential. Overall, the project delivered an integrated set of results linking carbon-sequestering cementitious materials, demountable connection design, and reusable composite interface behavior.