The development of scalable, sustainable energy harvesting technologies is central to Europe’s green and digital transition. Triboelectric nanogenerators offer a route to decentralised, low-cost energy generation from ambient motion, yet their adoption is limited by poor durability, complex fabrication, and reliance on fragile or unsustainable materials. This project has presented advances in three key areas: one, the creation of supply resilience as a key metric for electronic nanomaterials in Europe, identifying which materials are both high-performing and locally accessible, ensuring that the TENGs can be produced with European-sourced materials, two sustainable processing of carbon nanotubes and 2D materials in green solvents such as Cyrene, informing the formulation of printable, environmentally responsible nanomaterial inks, and three, engineering charge transport in 2D nanosheet networks, a critical bottleneck in triboelectric performance. Together, these works shape a vision for printable composite inks that are high-performing, scalable, and compatible with additive manufacturing. The project aims to demonstrate a fully printed TENG based on sustainable materials, highlighting its practical potential and broad impact across wearables, sensors, and mobility infrastructure.