Chemical Looping gAsification foR sustainAble production of biofuels

Rezultaty

Report on fate of tar surrogates on selected oxygen carriers

Results of tests in a batch fluidized bed reactor using tar surrogates together with oxidizing gases of steam and/or carbon dioxide as well as simulated gasification gas

Environmental risk assessment

Assessment of the environmental issues with respect to the fullscale biomasstoenduse chain development of plan for minimization of the negative environmental impact

Assessment of risks related to society

Assessment of the risks related to society with respect to the diffusion of full-scale biomass-to-end-use chains, development of plan for minimization of the risks related to society

Second public report

Summary of the major results obtained by the project within the preceding 12 months, made available for download on the website and sent by email to any interested stakeholder registered at the website

Strategies for biofuel deployment based on residuals

Calculation of overall costs and GHGemissions of relevant constellations of chain links under different boundary conditions by using a refined database development of scenarios up to 2050 using Technological Learning approaches

Forth public report

Summary of the major results obtained by the project within the preceding 15 months made available for download on the website and sent by email to any interested stakeholder registered at the website

Results of testing at up to 100 kWth scale using pre-treated straw

Demonstration of the feasibility of the CLG concept in two continuous reactors with a thermal input of 50 kWth CSIC and 100 kWth CTH with pretreated straw as feedstock results of parameter variations

Technology risk assessment

Assessmet of the risks related to technological development of the full process chain and development of a plan for possible technological risk mitigation

Techno-economic assessment of the full-scale biofuel production processes and applications

Interrelation and expandation of the technical and economic parameters for pretreatment gasification and fuel synthesis with data for feedstock supply quality and different distribution options modes distances storage to end users

Analysis of selected feedstock

Proximate analysis elemental analysis and determines ash composition ash fusibility for the selected types of feedstock ie wood pellets straw and residue from forestry

Health and safety risk assessment

Assessment of the health and safety issues with respect to the fullscale biomasstoenduse chain development of a plan for health and safety risk mitigation

Third public report

Summary of the major results obtained by the project within the preceding 15 months, made available for download on the website and sent by email to any interested stakeholder registered at the website

Results of testing at up to 100 kWth scale using wood chips/pellets

Demonstration of the feasibility of the CLG concept in two continuous reactors with a thermal input of 50 kWth (CSIC) and 100 kWth (CTH) with wood chips and forest residues as feedstock; results of parameter variations

Environmental evaluation of biofuel production processes via Life Cycle Analysis

Derivation of environmental performance indicators for each individual process units as part of the chain by a life cycle analysis LCA methodology calculation of environmental benefits generated in the production of biofuels by means of GHG emissions reduction

Economical risk assessment

Assessment of economic risks for the whole biomass to fuel process chain derivation of risk mitigation strategies to tackle the vulnerability amplified by the single chain links of the investigated biomasstoenduse constellations

Cost estimation for biomass feedstock supply

Analyses of costs of various categories of fuel supply; costs for pre-treated cereal straw derived from the experience with CENER’s pilot plant and up-scaling studies using previously developed pre-treatment simulation tools and economic models

First public report

Summary of the major results obtained by the project within the preceding 12 months, made available for download on the website and sent by email to any interested stakeholder registered at the website

Results of continuous testing with different fuels and oxygen carriers

Results of chemical looping gasification tests a 1.5 kWth reactor at CSIC and a 10 kWth reactor at CTH with several types of fresh and pre-treated biomass operated at different temperatures and gas flows; Selection of an oxygen carrier for pilot testing

Second public workshop

Organizaion of a public workshop to present the results of the project as annex to an international conference

Six monthly newsletters

Production of a newsletter giving news about project developments every six months and its dissemination to all relevant stakeholders who have registered their interest at the website

Publications

Presentions of the results of the project at international conferences and publications in peer-reviewed journals during the course of the project

First public workshop

Organization of public workshop to present the results of the project in Darmstadt – including a visit of the pilot test site

Logo and website

Creation of a project logo in order to create a recognizable view of the project’s vision and concept; creation of a fully interactive project website

Publikacje

Effects of Temperature, Operation Mode, and Steam Concentration on Alkali Release in Chemical Looping Conversion of Biomass─Experimental Investigation in a 10 kW<sub>th</sub> Pilot

Autorzy: Ivan Gogolev; Amir H. Soleimanisalim; Daofeng Mei; Anders Lyngfelt
Opublikowane w: Energy & Fuels (0887-0624) vol.In Press(2022), Numer 1, 2022, ISSN 0887-0624
Wydawca: American Chemical Society
DOI: 10.1021/acs.energyfuels.1c04353

Biomass chemical looping gasification for syngas production using LD Slag as oxygen carrier in a 1.5 kWth unit

Autorzy: Oscar Condori , Francisco García-Labiano *, Luis F. de Diego, María T. Izquierdo , Alberto Abad, Juan Ad ́ anez
Opublikowane w: Fuel Processing Technology, 2021, ISSN 0378-3820
Wydawca: Elsevier BV
DOI: 10.1016/j.fuproc.2021.106963

System Hydrodynamics of a 1 MWth Dual Circulating Fluidized Bed Chemical Looping Gasifier

Autorzy: Paul Dieringer; Falko Marx; Jochen Ströhle; Bernd Epple
Opublikowane w: Energies, Numer 1, 2023, ISSN 1996-1073
Wydawca: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/en16155630

Technoeconomic and Environmental Assessment of Biomass Chemical Looping Gasification for Advanced Biofuel Production

Autorzy: Valentina Gogulancea ,Angela Rolfe ,Mohammad Jaffar ,Caterina Brandoni ,Konstantinos Atsonios , Nikolaos Detsios,Paul Dieringer, Ye Huang
Opublikowane w: International Journal of Energy Research, 2023, ISSN 0363-907X
Wydawca: John Wiley & Sons Inc.
DOI: 10.1155/2023/6101270

Fate of ilmenite as oxygen carrier during 1 MWth chemical looping gasification of biogenic residues

Autorzy: Paul Dieringer Falko Marx Florian Lebendig Michael Müller Andrea Di Giuliano Katia Gallucci Jochen Ströhle Bernd Epple
Opublikowane w: Applications in Energy and Combustion Science, 2023, ISSN 2666-352X
Wydawca: Elsevier
DOI: 10.1016/j.jaecs.2023.100227

Assessment of the chemical looping gasification of wheat straw pellets at the 20 kWth scale

Autorzy: Oscar Condori; Alberto Abad; María T. Izquierdo; Luis F. de Diego; Francisco García-Labiano; Juan Adánez
Opublikowane w: Crossref, Numer 2, 2023, ISSN 0016-2361
Wydawca: Elsevier BV
DOI: 10.1016/j.fuel.2023.128059

Pretreated residual biomasses in fluidized beds for chemical looping gasification: Analysis of devolatilization data by statistical tools

Autorzy: Andrea Di Giuliano , Marta Gallucci , Barbara Malsegna , Stefania Lucantonio , Katia Gallucci*
Opublikowane w: Bioresource Technology Reports, 2022, ISSN 2589-014X
Wydawca: Elsevier
DOI: 10.1016/j.biteb.2021.100926

Study of defluidization of iron- and manganese-based oxygen carriers under highly reducing conditions in a lab-scale fluidized-bed batch reactor

Autorzy: Victor Purnomo, Duygu Yilmaz, Henrik Leion, Tobias Mattisson
Opublikowane w: Fuel Processing Technology, 2021, ISSN 0378-3820
Wydawca: Elsevier BV
DOI: 10.1016/j.fuproc.2021.106874

Solid flux measurement in dual fluidized bed processes based on solid samples

Autorzy: Falko Marx; Paul Dieringer; Jochen Ströhle; Bernd Epple
Opublikowane w: Crossref, Numer 3, 2023, ISSN 0016-2361
Wydawca: Elsevier BV
DOI: 10.1016/j.fuel.2023.127589

Effect of pre-treatment of herbaceous feedstocks on behavior of inorganic constituents under chemical looping gasification (CLG) conditions

Autorzy: Florian Lebendig; Michael Müller
Opublikowane w: Green chemistry 24(24), 9643-9658 (2022). doi:10.1039/D2GC02906E, Numer 5, 2023, ISSN 1463-9262
Wydawca: Royal Society of Chemistry
DOI: 10.1039/d2gc02906e

Devolatilization of Residual Biomasses for Chemical Looping Gasification in Fluidized Beds Made Up of Oxygen-Carriers

Autorzy: Andrea Di Giuliano; Stefania Lucantonio; Katia Gallucci
Opublikowane w: Energies, Vol 14, Iss 311, p 311 (2021), Numer 2, 2021, ISSN 1996-1073
Wydawca: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/en14020311

Experimental Evaluation of Manganese Ores for Chemical Looping Conversion of Synthetic Biomass Volatiles in a 300 W Reactor System

Autorzy: Ali Hedayati, Amir H. Soleimanisalim, Carl Johan Linderholm, Tobias Mattisson, Anders Lyngfe
Opublikowane w: Journal of Environmental Chemical Engineerin, 2021, ISSN 2213-3437
Wydawca: Elsevier BV
DOI: 10.1016/j.fuel.2021.122638

Effect of the Mass Conversion Degree of an Oxygen Carrier on Char Conversion and Its Implication for Chemical Looping Gasification.

Autorzy: Victor Purnomo; Daofeng Mei; Amir H. Soleimanisalim; Tobias Mattisson; Henrik Leion
Opublikowane w: Crossref, Numer 1, 2022, ISSN 0887-0624
Wydawca: American Chemical Society
DOI: 10.1021/acs.energyfuels.2c00944

Experimental assessments of pyrolytic and fluid-dynamic interactions between pretreated residual biomasses and fluidized beds made up of oxygen carriers for chemical looping gasification

Autorzy: Di Giuliano, A.; Malsegna, B.; Lucantonio, S.; Gallucci, K.
Opublikowane w: Crossref, Numer 2, 2023, ISSN 0921-8831
Wydawca: Elsevier BV
DOI: 10.1016/j.apt.2023.104010

Design of a 1 MWth Pilot Plant for Chemical Looping Gasification of Biogenic Residues

Autorzy: Falko Marx * , Paul Dieringer , Jochen Ströhle and Bernd Epple
Opublikowane w: Energies, 2021, ISSN 1996-1073
Wydawca: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/en14092581

Process efficiency and syngas quality from autothermal operation of a 1 MWth chemical looping gasifier with biogenic residues

Autorzy: Marx, Falko; Dieringer, Paul; Ströhle, Jochen; Epple, Bernd
Opublikowane w: Applications in Energy and Combustion Science, Numer 1, 2023, ISSN 2666-352X
Wydawca: Elsevier
DOI: 10.1016/j.jaecs.2023.100217

Design and control concept of a 1 MWth chemical looping gasifier allowing for efficient autothermal syngas production

Autorzy: Paul Dieringer; Falko Marx; Benjamin Michel; Jochen Ströhle; Bernd Epple
Opublikowane w: International Journal of Greenhouse Gas Control, Numer 1, 2023, ISSN 1750-5836
Wydawca: Elsevier BV
DOI: 10.1016/j.ijggc.2023.103929

Review on dynamic process modeling of gasification based biorefineries and bio-based heat & power plants

Autorzy: Konstantinos Atsonios, Athanasios Nesiadis, Nikolaos Detsios, Konstantina Koutita, Nikos Nikolopoulos, Panagiotis Grammelis
Opublikowane w: Fuel Processing Technology, Numer 197, 2020, Strona(/y) 106188, ISSN 0378-3820
Wydawca: Elsevier BV
DOI: 10.1016/j.fuproc.2019.106188

Process Control Strategies in Chemical Looping Gasification—A Novel Process for the Production of Biofuels Allowing for Net Negative CO2 Emissions

Autorzy: Paul Dieringer, Falko Marx, Falah Alobaid, Jochen Ströhle, Bernd Epple
Opublikowane w: Applied Sciences, Numer 10/12, 2020, Strona(/y) 4271, ISSN 2076-3417
Wydawca: MDPI
DOI: 10.3390/app10124271

Investigations on the Effect of Pre-Treatment of Wheat Straw on Ash-Related Issues in Chemical Looping Gasification (CLG) in Comparison with Woody Biomass

Autorzy: F. Lebendig, I. Funcia, R. Pérez-Vega, M. Müller
Opublikowane w: Energies, 2022, ISSN 1996-1073
Wydawca: Multidisciplinary Digital Publishing Institute (MDPI)
DOI: 10.3390/en15093422

Novel Application of Pretreatment and Diagnostic Method Using Dynamic Pressure Fluctuations to Resolve and Detect Issues Related to Biogenic Residue Ash in Chemical Looping Gasification

Autorzy: Andrea Di Giuliano; Ibai Funcia; Raúl Pérez-Vega; Javier Gil; Katia Gallucci
Opublikowane w: Volume 8, Numer 2, 2020, ISSN 2227-9717
Wydawca: MDPI
DOI: 10.3390/pr8091137

Influences of the Pretreatments of Residual Biomass on Gasification Processes: Experimental Devolatilizations Study in a Fluidized Bed

Autorzy: Stefania Lucantonio; Andrea Di Giuliano; Katia Gallucci
Opublikowane w: Numer 12, Numer 2, 2021, ISSN 2076-3417
Wydawca: MDPI
DOI: 10.3390/app11125722

Thermochemical conversion of biomass volatiles via chemical looping: Comparison of ilmenite and steel converter waste materials as oxygen carriers

Autorzy: Ali Hedayati; Amir H. Soleimanisalim; Tobias Mattisson; Anders Lyngfelt
Opublikowane w: Fuel, Numer 1, 2022, ISSN 0016-2361
Wydawca: Elsevier BV
DOI: 10.1016/j.fuel.2021.122638

Biomass chemical looping gasification for syngas production using ilmenite as oxygen carrier in a 1.5 kWth unit

Autorzy: Oscar Condori; Francisco García-Labiano; Luis F. de Diego; Maria Izquierdo; Alberto Abad; Juan Adánez
Opublikowane w: Chemical Engineering Journal, Numer 6, 2021, ISSN 1385-8947
Wydawca: Elsevier BV
DOI: 10.1016/j.cej.2020.126679

Syngas production in a 1.5 kWth biomass chemical looping gasification unit using Fe and Mn ores as the oxygen carrier

Autorzy: Oscar Condori; Luis F. de Diego; Francisco García-Labiano; Maria Izquierdo; Alberto Abad; Juan Adánez
Opublikowane w: Energy & Fuels, Numer 2, 2021, ISSN 1520-5029
Wydawca: ACS Publications
DOI: 10.1021/acs.energyfuels.1c01878

Pretreated residual biomasses in fluidized beds for chemical looping Gasification: Experimental devolatilizations and characterization of ashes behavior

Autorzy: Andrea Di Giuliano; Stefania Lucantonio; Barbara Malsegna; Katia Gallucci
Opublikowane w: Crossref, Numer 2, 2022, ISSN 0960-8524
Wydawca: Elsevier BV
DOI: 10.1016/j.biortech.2021.126514

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